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Title: Hot excitons are responsible for increasing photoluminescence blinking activity in single lead sulfide/cadmium sulfide nanocrystals

The kinetics of PL blinking for isolated PbS/CdS nanocrystals changes with the photon excitation energy, with PL blinking increasing in frequency and changing from a two-state to a multistate on/off switching when the excitation energy changes from 1S h–1S e(≈1.4 eV) to 1P h–1P e(≈2.4 eV).
Authors:
ORCiD logo [1] ;  [2] ;  [2] ; ORCiD logo [2]
  1. Brookhaven National Lab. (BNL), Upton, NY (United States); Stony Brook Univ., NY (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
Publication Date:
Report Number(s):
BNL-114847-2017-JAAM
Journal ID: ISSN 1359-7345; CHCOFS
Grant/Contract Number:
SC0012704
Type:
Accepted Manuscript
Journal Name:
ChemComm
Additional Journal Information:
Journal Volume: 54; Journal Issue: 5; Journal ID: ISSN 1359-7345
Publisher:
Royal Society of Chemistry
Research Org:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE
OSTI Identifier:
1425016

Chen, Jia-Shiang, Zang, Huidong, Li, Mingxing, and Cotlet, Mircea. Hot excitons are responsible for increasing photoluminescence blinking activity in single lead sulfide/cadmium sulfide nanocrystals. United States: N. p., Web. doi:10.1039/C7CC08356D.
Chen, Jia-Shiang, Zang, Huidong, Li, Mingxing, & Cotlet, Mircea. Hot excitons are responsible for increasing photoluminescence blinking activity in single lead sulfide/cadmium sulfide nanocrystals. United States. doi:10.1039/C7CC08356D.
Chen, Jia-Shiang, Zang, Huidong, Li, Mingxing, and Cotlet, Mircea. 2017. "Hot excitons are responsible for increasing photoluminescence blinking activity in single lead sulfide/cadmium sulfide nanocrystals". United States. doi:10.1039/C7CC08356D.
@article{osti_1425016,
title = {Hot excitons are responsible for increasing photoluminescence blinking activity in single lead sulfide/cadmium sulfide nanocrystals},
author = {Chen, Jia-Shiang and Zang, Huidong and Li, Mingxing and Cotlet, Mircea},
abstractNote = {The kinetics of PL blinking for isolated PbS/CdS nanocrystals changes with the photon excitation energy, with PL blinking increasing in frequency and changing from a two-state to a multistate on/off switching when the excitation energy changes from 1Sh–1Se(≈1.4 eV) to 1Ph–1Pe(≈2.4 eV).},
doi = {10.1039/C7CC08356D},
journal = {ChemComm},
number = 5,
volume = 54,
place = {United States},
year = {2017},
month = {12}
}