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Title: Single-shot terahertz time-domain spectroscopy in pulsed high magnetic fields

Abstract

Here, we have developed a single-shot terahertz time-domain spectrometer to perform optical-pump/terahertz-probe experiments in pulsed, high magnetic fields up to 30 T. The single-shot detection scheme for measuring a terahertz waveform incorporates a reflective echelon to create time-delayed beamlets across the intensity profile of the optical gate beam before it spatially and temporally overlaps with the terahertz radiation in a ZnTe detection crystal. After imaging the gate beam onto a camera, we can retrieve the terahertz time-domain waveform by analyzing the resulting image. To demonstrate the utility of our technique, we measured cyclotron resonance absorption of optically excited carriers in the terahertz frequency range in intrinsic silicon at high magnetic fields, with results that agree well with published values.

Authors:
 [1];  [2];  [1];  [1];  [1];  [1];  [1];  [3];  [1];  [4];  [5];  [2];  [1]
+ Show Author Affiliations
  1. Rice Univ., Houston, TX (United States)
  2. Yokohama National Univ., Yokohama (Japan)
  3. The Univ. of Tokyo, Tokyo (Japan)
  4. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  5. Tohoku Univ., Sendai (Japan)
Publication Date:
Research Org.:
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1352155
Grant/Contract Number:  
DMR-1310138
Resource Type:
Accepted Manuscript
Journal Name:
Optics Express
Additional Journal Information:
Journal Volume: 24; Journal Issue: 26; Journal ID: ISSN 1094-4087
Publisher:
Optical Society of America (OSA)
Country of Publication:
United States
Language:
English
Subject:
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS; magneto-optic systems; spectroscopy; terahertz

Citation Formats

Noe, II, G. Timothy, Katayama, Ikufumi, Katsutani, Fumiya, Allred, James J., Horowitz, Jeffrey A., Sullivan, David M., Zhang, Qi, Sekiguchi, Fumiya, Woods, Gary L., Hoffmann, Matthias C., Nojiri, Hiroyuki, Takeda, Jun, and Kono, Junichiro. Single-shot terahertz time-domain spectroscopy in pulsed high magnetic fields. United States: N. p., 2016. Web. doi:10.1364/oe.24.030328.
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Noe, II, G. Timothy, Katayama, Ikufumi, Katsutani, Fumiya, Allred, James J., Horowitz, Jeffrey A., Sullivan, David M., Zhang, Qi, Sekiguchi, Fumiya, Woods, Gary L., Hoffmann, Matthias C., Nojiri, Hiroyuki, Takeda, Jun, & Kono, Junichiro. Single-shot terahertz time-domain spectroscopy in pulsed high magnetic fields. United States. https://doi.org/10.1364/oe.24.030328
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Noe, II, G. Timothy, Katayama, Ikufumi, Katsutani, Fumiya, Allred, James J., Horowitz, Jeffrey A., Sullivan, David M., Zhang, Qi, Sekiguchi, Fumiya, Woods, Gary L., Hoffmann, Matthias C., Nojiri, Hiroyuki, Takeda, Jun, and Kono, Junichiro. Thu . "Single-shot terahertz time-domain spectroscopy in pulsed high magnetic fields". United States. https://doi.org/10.1364/oe.24.030328. https://www.osti.gov/servlets/purl/1352155.
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@article{osti_1352155,
title = {Single-shot terahertz time-domain spectroscopy in pulsed high magnetic fields},
author = {Noe, II, G. Timothy and Katayama, Ikufumi and Katsutani, Fumiya and Allred, James J. and Horowitz, Jeffrey A. and Sullivan, David M. and Zhang, Qi and Sekiguchi, Fumiya and Woods, Gary L. and Hoffmann, Matthias C. and Nojiri, Hiroyuki and Takeda, Jun and Kono, Junichiro},
abstractNote = {Here, we have developed a single-shot terahertz time-domain spectrometer to perform optical-pump/terahertz-probe experiments in pulsed, high magnetic fields up to 30 T. The single-shot detection scheme for measuring a terahertz waveform incorporates a reflective echelon to create time-delayed beamlets across the intensity profile of the optical gate beam before it spatially and temporally overlaps with the terahertz radiation in a ZnTe detection crystal. After imaging the gate beam onto a camera, we can retrieve the terahertz time-domain waveform by analyzing the resulting image. To demonstrate the utility of our technique, we measured cyclotron resonance absorption of optically excited carriers in the terahertz frequency range in intrinsic silicon at high magnetic fields, with results that agree well with published values.},
doi = {10.1364/oe.24.030328},
journal = {Optics Express},
number = 26,
volume = 24,
place = {United States},
year = {Thu Dec 22 00:00:00 EST 2016},
month = {Thu Dec 22 00:00:00 EST 2016}
}
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https://doi.org/10.1364/oe.24.030328
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Terahertz cyclotron resonance spectroscopy of an AlGaN/GaN heterostructure using a high-field pulsed magnet and an asynchronous optical sampling technique
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    Works referencing / citing this record:

    Corrective re-gridding techniques for non-uniform sampling in time-domain terahertz spectroscopy
    journal, January 2019

    • Potts, A. M.; Mai, T. T.; Warren, M. T.
    • Journal of the Optical Society of America B, Vol. 36, Issue 4
    • DOI: 10.1364/josab.36.001037

    Toward quasi-DC conductivity of warm dense matter measured by single-shot terahertz spectroscopy
    journal, October 2018

    • Ofori-Okai, B. K.; Descamps, A.; Lu, J.
    • Review of Scientific Instruments, Vol. 89, Issue 10
    • DOI: 10.1063/1.5038944

    Broadband ultrafast terahertz spectroscopy in the 25 T Split Florida-Helix
    journal, July 2018

    • Curtis, Jeremy A.; Burch, Ashlyn D.; Barman, Biplob
    • Review of Scientific Instruments, Vol. 89, Issue 7
    • DOI: 10.1063/1.5023384

    Terahertz Faraday and Kerr rotation spectroscopy of Bi 1 − x Sb x films in high magnetic fields up to 30 tesla
    journal, September 2019

    An echelon-based single shot optical and terahertz Kerr effect spectrometer
    journal, May 2019

    • Mead, Griffin; Katayama, Ikufumi; Takeda, Jun
    • Review of Scientific Instruments, Vol. 90, Issue 5
    • DOI: 10.1063/1.5088377

    An Echelon-Based Single shot Optical and Terahertz kerr Effect Spectrometer
    conference, June 2019

    • Mead, Griffin; Blake, Geoffrey
    • Proceedings of the 74th International Symposium on Molecular Spectroscopy
    • DOI: 10.15278/isms.2019.mj06
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