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Title: Electron doping evolution of the magnetic excitations in NaFe1-xCoxAs

Abstract

We use time-of-flight (TOF) inelastic neutron scattering (INS) spectroscopy to investigate the doping dependence of magnetic excitations across the phase diagram of NaFe1-xCoxAs with x = 0, 0.0175, 0.0215, 0.05, and 0.11. The effect of electron-doping by partially substituting Fe by Co is to form resonances that couple with superconductivity, broaden and suppress low energy (E 80 meV) spin excitations compared with spin waves in undoped NaFeAs. However, high energy (E > 80 meV) spin excitations are weakly Co-doping dependent. Integration of the local spin dynamic susceptibility "(!) of NaFe1-xCoxAs reveals a total fluctuating moment of 3.6 μ2 B/Fe and a small but systematic reduction with electron doping. The presence of a large spin gap in the Cooverdoped nonsuperconducting NaFe0.89Co0.11As suggests that Fermi surface nesting is responsible for low-energy spin excitations. These results parallel Ni-doping evolution of spin excitations in BaFe2-xNixAs2, confirming the notion that low-energy spin excitations coupling with itinerant electrons are important for superconductivity, while weakly doping dependent high-energy spin excitations result from localized moments.

Authors:
 [1];  [1];  [1];  [2];  [1];  [3];  [3];  [3];  [4];  [1]
  1. Rice Univ., Houston, TX (United States)
  2. Beijing Normal Univ. (China)
  3. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  4. ISIS Facility, Rutherford Appleton Laboratory
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). High Flux Isotope Reactor (HFIR); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1261361
Alternate Identifier(s):
OSTI ID: 1256786
Grant/Contract Number:  
AC05-00OR22725; SC0012311
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 93; Journal Issue: 21; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Carr, Scott V., Zhang, Chenglin, Song, Yu, Tan, Guotai, Li, Yu, Abernathy, Douglas L., Stone, Matthew B., Granroth, Garrett E., Perring, T. G., and Dai, Pengcheng. Electron doping evolution of the magnetic excitations in NaFe1-xCoxAs. United States: N. p., 2016. Web. doi:10.1103/PhysRevB.93.214506.
Carr, Scott V., Zhang, Chenglin, Song, Yu, Tan, Guotai, Li, Yu, Abernathy, Douglas L., Stone, Matthew B., Granroth, Garrett E., Perring, T. G., & Dai, Pengcheng. Electron doping evolution of the magnetic excitations in NaFe1-xCoxAs. United States. doi:10.1103/PhysRevB.93.214506.
Carr, Scott V., Zhang, Chenglin, Song, Yu, Tan, Guotai, Li, Yu, Abernathy, Douglas L., Stone, Matthew B., Granroth, Garrett E., Perring, T. G., and Dai, Pengcheng. Mon . "Electron doping evolution of the magnetic excitations in NaFe1-xCoxAs". United States. doi:10.1103/PhysRevB.93.214506. https://www.osti.gov/servlets/purl/1261361.
@article{osti_1261361,
title = {Electron doping evolution of the magnetic excitations in NaFe1-xCoxAs},
author = {Carr, Scott V. and Zhang, Chenglin and Song, Yu and Tan, Guotai and Li, Yu and Abernathy, Douglas L. and Stone, Matthew B. and Granroth, Garrett E. and Perring, T. G. and Dai, Pengcheng},
abstractNote = {We use time-of-flight (TOF) inelastic neutron scattering (INS) spectroscopy to investigate the doping dependence of magnetic excitations across the phase diagram of NaFe1-xCoxAs with x = 0, 0.0175, 0.0215, 0.05, and 0.11. The effect of electron-doping by partially substituting Fe by Co is to form resonances that couple with superconductivity, broaden and suppress low energy (E 80 meV) spin excitations compared with spin waves in undoped NaFeAs. However, high energy (E > 80 meV) spin excitations are weakly Co-doping dependent. Integration of the local spin dynamic susceptibility "(!) of NaFe1-xCoxAs reveals a total fluctuating moment of 3.6 μ2 B/Fe and a small but systematic reduction with electron doping. The presence of a large spin gap in the Cooverdoped nonsuperconducting NaFe0.89Co0.11As suggests that Fermi surface nesting is responsible for low-energy spin excitations. These results parallel Ni-doping evolution of spin excitations in BaFe2-xNixAs2, confirming the notion that low-energy spin excitations coupling with itinerant electrons are important for superconductivity, while weakly doping dependent high-energy spin excitations result from localized moments.},
doi = {10.1103/PhysRevB.93.214506},
journal = {Physical Review B},
number = 21,
volume = 93,
place = {United States},
year = {2016},
month = {6}
}

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