Toughness and strength of nanocrystalline graphene
Abstract
Pristine monocrystalline graphene is claimed to be the strongest material known with remarkable mechanical and electrical properties. However, graphene made with scalable fabrication techniques is polycrystalline and contains inherent nanoscale line and point defects—grain boundaries and grain-boundary triple junctions—that lead to significant statistical fluctuations in toughness and strength. These fluctuations become particularly pronounced for nanocrystalline graphene where the density of defects is high. Here we use large-scale simulation and continuum modelling to show that the statistical variation in toughness and strength can be understood with ‘weakest-link’ statistics. We develop the first statistical theory of toughness in polycrystalline graphene, and elucidate the nanoscale origins of the grain-size dependence of its strength and toughness. Lastly, our results should lead to more reliable graphene device design, and provide a framework to interpret experimental results in a broad class of two-dimensional materials.
- Authors:
-
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California, Berkeley, CA (United States); Miller Institute for Basic Research in Science, Berkeley, CA (United States)
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California, Berkeley, CA (United States)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1255548
- Alternate Identifier(s):
- OSTI ID: 1415954
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 7; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Shekhawat, Ashivni, and Ritchie, Robert O. Toughness and strength of nanocrystalline graphene. United States: N. p., 2016.
Web. doi:10.1038/ncomms10546.
Shekhawat, Ashivni, & Ritchie, Robert O. Toughness and strength of nanocrystalline graphene. United States. https://doi.org/10.1038/ncomms10546
Shekhawat, Ashivni, and Ritchie, Robert O. Thu .
"Toughness and strength of nanocrystalline graphene". United States. https://doi.org/10.1038/ncomms10546. https://www.osti.gov/servlets/purl/1255548.
@article{osti_1255548,
title = {Toughness and strength of nanocrystalline graphene},
author = {Shekhawat, Ashivni and Ritchie, Robert O.},
abstractNote = {Pristine monocrystalline graphene is claimed to be the strongest material known with remarkable mechanical and electrical properties. However, graphene made with scalable fabrication techniques is polycrystalline and contains inherent nanoscale line and point defects—grain boundaries and grain-boundary triple junctions—that lead to significant statistical fluctuations in toughness and strength. These fluctuations become particularly pronounced for nanocrystalline graphene where the density of defects is high. Here we use large-scale simulation and continuum modelling to show that the statistical variation in toughness and strength can be understood with ‘weakest-link’ statistics. We develop the first statistical theory of toughness in polycrystalline graphene, and elucidate the nanoscale origins of the grain-size dependence of its strength and toughness. Lastly, our results should lead to more reliable graphene device design, and provide a framework to interpret experimental results in a broad class of two-dimensional materials.},
doi = {10.1038/ncomms10546},
journal = {Nature Communications},
number = ,
volume = 7,
place = {United States},
year = {Thu Jan 28 00:00:00 EST 2016},
month = {Thu Jan 28 00:00:00 EST 2016}
}
Web of Science
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- Nanoscale, Vol. 8, Issue 12
Grain size and hydroxyl-coverage dependent tribology of polycrystalline graphene
journal, July 2019
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Evidence of a two-dimensional glass transition in graphene: Insights from molecular simulations
journal, March 2019
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Sliding Over Graphene Grain Boundaries: A Step Towards Macroscale Superlubricity
preprint, January 2020
- Gao, Xiang; Ouyang, Wengen; Hod, Oded
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Superb electromagnetic wave-absorbing composites based on large-scale graphene and carbon nanotube films
journal, May 2017
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Infusion of Graphene Quantum Dots to Create Stronger, Tougher, and Brighter Polymer Composites
journal, August 2017
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A Review on Brittle Fracture Nanomechanics by All-Atom Simulations
journal, July 2019
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Elastic straining of free-standing monolayer graphene
journal, January 2020
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Revealing the 3D structure of graphene defects
journal, September 2018
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Mechanical properties of atomically thin boron nitride and the role of interlayer interactions
journal, June 2017
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A review on graphene-based polymer composite coatings for the corrosion protection of metals
journal, August 2019
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Food Intake Depression and Other Metabolic Effects of Tannic Acid in the Rat
journal, May 1970
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Stretchability of PMMA-supported CVD graphene and of its electrical contacts
journal, October 2019
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