Examining the influence of grain size on radiation tolerance in the nanocrystalline regime
Abstract
Here, nanocrystalline materials have been proposed as superior radiation tolerant materials in comparison to coarse grain counterparts. However, there is still a limited understanding whether a particular nanocrystalline grain size is required to obtain significant improvements in key deleterious effects resulting from energetic irradiation. This work employs the use of in-situ heavy ion irradiation transmission electron microscopy experiments coupled with quantitative defect characterization and precession electron diffraction to explore the sensitivity of defect size and density within the nanocrystalline regime in platinum. Under the explored experimental conditions, no significant change in either the defect size or density between grain sizes of 20 and 100 nm was observed. Furthermore, the in-situ transmission electron microscopy irradiations illustrate stable sessile defect clusters of 1-3 nm adjacent to most grain boundaries, which are traditionally treated as strong defect sinks. The stability of these sessile defects observed in-situ in small, 20-40 nm, grains is the proposed primary mechanism for a lack of defect density trends. Lastly, this scaling breakdown in radiation improvement with decreasing grain size has practical importance on nanoscale grain boundary engineering approaches for proposed radiation tolerant alloys.
- Authors:
-
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States). Material, Physical, and Chemical Sciences
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1479967
- Alternate Identifier(s):
- OSTI ID: 1435481; OSTI ID: 1441471
- Report Number(s):
- LA-UR-18-29343; SAND-2018-4283J
Journal ID: ISSN 0003-6951
- Grant/Contract Number:
- AC04-94AL85000; AC52-06NA25396; NA0003525
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Applied Physics Letters
- Additional Journal Information:
- Journal Volume: 112; Journal Issue: 18; Journal ID: ISSN 0003-6951
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 77 NANOSCIENCE AND NANOTECHNOLOGY
Citation Formats
Barr, Christopher M., Li, Nan, Boyce, Brad L., and Hattar, Khalid. Examining the influence of grain size on radiation tolerance in the nanocrystalline regime. United States: N. p., 2018.
Web. doi:10.1063/1.5016822.
Barr, Christopher M., Li, Nan, Boyce, Brad L., & Hattar, Khalid. Examining the influence of grain size on radiation tolerance in the nanocrystalline regime. United States. https://doi.org/10.1063/1.5016822
Barr, Christopher M., Li, Nan, Boyce, Brad L., and Hattar, Khalid. Mon .
"Examining the influence of grain size on radiation tolerance in the nanocrystalline regime". United States. https://doi.org/10.1063/1.5016822. https://www.osti.gov/servlets/purl/1479967.
@article{osti_1479967,
title = {Examining the influence of grain size on radiation tolerance in the nanocrystalline regime},
author = {Barr, Christopher M. and Li, Nan and Boyce, Brad L. and Hattar, Khalid},
abstractNote = {Here, nanocrystalline materials have been proposed as superior radiation tolerant materials in comparison to coarse grain counterparts. However, there is still a limited understanding whether a particular nanocrystalline grain size is required to obtain significant improvements in key deleterious effects resulting from energetic irradiation. This work employs the use of in-situ heavy ion irradiation transmission electron microscopy experiments coupled with quantitative defect characterization and precession electron diffraction to explore the sensitivity of defect size and density within the nanocrystalline regime in platinum. Under the explored experimental conditions, no significant change in either the defect size or density between grain sizes of 20 and 100 nm was observed. Furthermore, the in-situ transmission electron microscopy irradiations illustrate stable sessile defect clusters of 1-3 nm adjacent to most grain boundaries, which are traditionally treated as strong defect sinks. The stability of these sessile defects observed in-situ in small, 20-40 nm, grains is the proposed primary mechanism for a lack of defect density trends. Lastly, this scaling breakdown in radiation improvement with decreasing grain size has practical importance on nanoscale grain boundary engineering approaches for proposed radiation tolerant alloys.},
doi = {10.1063/1.5016822},
journal = {Applied Physics Letters},
number = 18,
volume = 112,
place = {United States},
year = {Mon Apr 30 00:00:00 EDT 2018},
month = {Mon Apr 30 00:00:00 EDT 2018}
}
Web of Science
Works referenced in this record:
Materials challenges in nuclear energy
journal, February 2013
- Zinkle, S. J.; Was, G. S.
- Acta Materialia, Vol. 61, Issue 3
Calculated grain size-dependent vacancy supersaturation and its effect on void formation
journal, April 1974
- Singh, B. N.; Foreman, A. J. E.
- Philosophical Magazine, Vol. 29, Issue 4
Probing grain boundary sink strength at the nanoscale: Energetics and length scales of vacancy and interstitial absorption by grain boundaries in -Fe
journal, February 2012
- Tschopp, M. A.; Solanki, K. N.; Gao, F.
- Physical Review B, Vol. 85, Issue 6
Efficient Annealing of Radiation Damage Near Grain Boundaries via Interstitial Emission
journal, March 2010
- Bai, X. M.; Voter, A. F.; Hoagland, R. G.
- Science, Vol. 327, Issue 5973
Second Paper on Statistics Associated with the Random Disorientation of Cubes
journal, January 1958
- Mackenzie, J. K.
- Biometrika, Vol. 45, Issue 1-2
Radiation damage in helium ion irradiated nanocrystalline Fe
journal, June 2012
- Yu, K. Y.; Liu, Y.; Sun, C.
- Journal of Nuclear Materials, Vol. 425, Issue 1-3
Study of defect evolution by TEM with in situ ion irradiation and coordinated modeling
journal, June 2012
- Li, Meimei; Kirk, M. A.; Baldo, P. M.
- Philosophical Magazine, Vol. 92, Issue 16
Grain size effect on radiation tolerance of nanocrystalline Mo
journal, October 2016
- Cheng, G. M.; Xu, W. Z.; Wang, Y. Q.
- Scripta Materialia, Vol. 123
Heterogeneous dislocation formation and solute redistribution near grain boundaries in austenitic stainless steel under electron irradiation
journal, April 2001
- Sakaguchi, N.; Watanabe, S.; Takahashi, H.
- Acta Materialia, Vol. 49, Issue 7
Study of rapid grain boundary migration in a nanocrystalline Ni thin film
journal, January 2011
- Kacher, Josh; Robertson, I. M.; Nowell, Matt
- Materials Science and Engineering: A, Vol. 528, Issue 3
Defect-interface interactions
journal, October 2015
- Beyerlein, I. J.; Demkowicz, M. J.; Misra, A.
- Progress in Materials Science, Vol. 74
Unraveling irradiation induced grain growth with in situ transmission electron microscopy and coordinated modeling
journal, November 2015
- Bufford, D. C.; Abdeljawad, F. F.; Foiles, S. M.
- Applied Physics Letters, Vol. 107, Issue 19
Diffusivity and permeability of hydrogen in neutron irradiated molybdenum and platinum
journal, April 1983
- Katsuta, H.; Iwai, T.; Ohno, H.
- Journal of Nuclear Materials, Vol. 115, Issue 2-3
Computer Simulation of Displacement Cascades in Nanocrystalline Ni
journal, March 2002
- Samaras, M.; Derlet, P. M.; Van Swygenhoven, H.
- Physical Review Letters, Vol. 88, Issue 12
In situ Evidence of Defect Cluster Absorption by Grain Boundaries in Kr Ion Irradiated Nanocrystalline Ni
journal, February 2013
- Sun, C.; Song, M.; Yu, K. Y.
- Metallurgical and Materials Transactions A, Vol. 44, Issue 4
Helium bubble nucleation at grain boundaries
journal, December 1983
- Lane, P. L.; Goodhew, P. J.
- Philosophical Magazine A, Vol. 48, Issue 6
Softening of nanocrystalline metals at very small grain sizes
journal, February 1998
- Schiøtz, Jakob; Di Tolla, Francesco D.; Jacobsen, Karsten W.
- Nature, Vol. 391, Issue 6667
Heavy-ion irradiations of Fe and Fe–Cr model alloys Part 2: Damage evolution in thin-foils at higher doses
journal, July 2008
- Hernández-Mayoral, M.; Yao, Z.; Jenkins, M. L.
- Philosophical Magazine, Vol. 88, Issue 21
Impact of irradiation on the microstructure of nanocrystalline materials
journal, August 2004
- Nita, N.; Schaeublin, R.; Victoria, M.
- Journal of Nuclear Materials, Vol. 329-333
SRIM – The stopping and range of ions in matter (2010)
journal, June 2010
- Ziegler, James F.; Ziegler, M. D.; Biersack, J. P.
- Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 268, Issue 11-12
Atomic scale modelling of the primary damage state of irradiated fcc and bcc nanocrystalline metals
journal, June 2006
- Samaras, M.; Derlet, P. M.; Swygenhoven, H. Van
- Journal of Nuclear Materials, Vol. 351, Issue 1-3
Analysis of damage curves — a key for understanding point-defect properties in platinum
journal, February 1978
- Frank, W.; Seeger, A.
- Journal of Nuclear Materials, Vol. 69-70
Role of atomic structure on grain boundary-defect interactions in Cu
journal, June 2012
- Bai, Xian-Ming; Vernon, Louis J.; Hoagland, Richard G.
- Physical Review B, Vol. 85, Issue 21
Radiation damage near grain boundaries
journal, October 2003
- Samaras, M.; Derlet, P. M.; Van Swygenhoven†, H.
- Philosophical Magazine, Vol. 83, Issue 31-34
Evidence of a temperature transition for denuded zone formation in nanocrystalline Fe under He irradiation
journal, October 2016
- El-Atwani, O.; Nathaniel II, J. E.; Leff, A. C.
- Materials Research Letters
A thermal spike model of grain growth under irradiation
journal, January 2008
- Kaoumi, D.; Motta, A. T.; Birtcher, R. C.
- Journal of Applied Physics, Vol. 104, Issue 7
In situ studies on radiation tolerance of nanotwinned Cu
journal, June 2016
- Chen, Y.; Li, J.; Yu, K. Y.
- Acta Materialia, Vol. 111
Mobility and coalescence of stacking fault tetrahedra in Cu
journal, March 2015
- Martínez, Enrique; Uberuaga, Blas P.
- Scientific Reports, Vol. 5, Issue 1
In situ probing of the evolution of irradiation-induced defects in copper
journal, August 2013
- Li, N.; Hattar, K.; Misra, A.
- Journal of Nuclear Materials, Vol. 439, Issue 1-3
Void Volume Swelling dependent on Grain Size in an Austenitic Stainless Steel
journal, August 1973
- Singh, B. N.
- Nature Physical Science, Vol. 244, Issue 139
Radiation resistance of nano-crystalline iron: Coupling of the fundamental segregation process and the annihilation of interstitials and vacancies near the grain boundaries
journal, May 2016
- Li, Xiangyan; Liu, Wei; Xu, Yichun
- Acta Materialia, Vol. 109
Effect of grain boundary character on sink efficiency
journal, October 2012
- Han, W. Z.; Demkowicz, M. J.; Fu, E. G.
- Acta Materialia, Vol. 60, Issue 18
Design of Radiation Tolerant Materials Via Interface Engineering
journal, September 2013
- Han, Weizhong; Demkowicz, Michael J.; Mara, Nathan A.
- Advanced Materials, Vol. 25, Issue 48
Instability of irradiation induced defects in nanostructured materials
journal, May 1997
- Rose, M.; Balogh, A. G.; Hahn, H.
- Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 127-128
The role of grain size in He bubble formation: Implications for swelling resistance
journal, February 2017
- El-Atwani, O.; Nathaniel, J. E.; Leff, A. C.
- Journal of Nuclear Materials, Vol. 484
In-situ TEM observation of the response of ultrafine- and nanocrystalline-grained tungsten to extreme irradiation environments
journal, May 2014
- El-Atwani, O.; Hinks, J. A.; Greaves, G.
- Scientific Reports, Vol. 4, Issue 1
Helium bubble formation in ultrafine and nanocrystalline tungsten under different extreme conditions
journal, March 2015
- El-Atwani, O.; Hattar, K.; Hinks, J. A.
- Journal of Nuclear Materials, Vol. 458
The relationship between grain boundary structure, defect mobility and grain boundary sink efficiency
journal, March 2015
- Uberuaga, Blas Pedro; Vernon, Louis J.; Martinez, Enrique
- Scientific Reports, Vol. 5, Issue 1
Incoherent twin boundary migration induced by ion irradiation in Cu
journal, January 2013
- Li, N.; Wang, J.; Wang, Y. Q.
- Journal of Applied Physics, Vol. 113, Issue 2
Direct Observation of Sink-Dependent Defect Evolution in Nanocrystalline Iron under Irradiation
journal, May 2017
- El-Atwani, O.; Nathaniel, J. E.; Leff, A. C.
- Scientific Reports, Vol. 7, Issue 1
In Situ Study of Defect Migration Kinetics and Self-Healing of Twin Boundaries in Heavy Ion Irradiated Nanotwinned Metals
journal, April 2015
- Li, J.; Yu, K. Y.; Chen, Y.
- Nano Letters, Vol. 15, Issue 5
Accumulation and recovery of defects in ion-irradiated nanocrystalline gold
journal, September 2001
- Chimi, Y.; Iwase, A.; Ishikawa, N.
- Journal of Nuclear Materials, Vol. 297, Issue 3
Irradiation damage of single crystal, coarse-grained, and nanograined copper under helium bombardment at 450 °C
journal, October 2013
- Han, Weizhong; Fu, E. G.; Demkowicz, Michael J.
- Journal of Materials Research, Vol. 28, Issue 20
Concurrent in situ ion irradiation transmission electron microscope
journal, November 2014
- Hattar, K.; Bufford, D. C.; Buller, D. L.
- Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 338
On the use of SRIM for computing radiation damage exposure
journal, September 2013
- Stoller, R. E.; Toloczko, M. B.; Was, G. S.
- Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 310
Effect of Grain Boundary Stresses on Sink Strength
journal, November 2013
- Jiang, Chao; Swaminathan, Narasimhan; Deng, Jie
- Materials Research Letters, Vol. 2, Issue 2
Thermal and fission neutron-produced defect configurations in platinum
journal, February 1978
- Coltman, R. R.; Klabunde, C. E.; Redman, J. K.
- Journal of Nuclear Materials, Vol. 69-70
Evolution of fine-scale defects in stainless steels neutron-irradiated at 275 °C
journal, April 2003
- Edwards, D. J.; Simonen, E. P.; Bruemmer, S. M.
- Journal of Nuclear Materials, Vol. 317, Issue 1
In situ Transmission Electron Microscopy He+ implantation and thermal aging of nanocrystalline iron
journal, December 2016
- Muntifering, Brittany; Fang, Youwu; Leff, Asher C.
- Journal of Nuclear Materials, Vol. 482
Recovery of irradiated and quenched metals
journal, February 1973
- Schilling, W.; Sonnenberg, K.
- Journal of Physics F: Metal Physics, Vol. 3, Issue 2
Grain boundary related effects in aluminium during 600 MeV proton irradiation at different temperatures
journal, May 1984
- Singh, B. N.; Leffers, T.; Green, W. V.
- Journal of Nuclear Materials, Vol. 122, Issue 1-3
Dynamic interaction between grain boundary and stacking fault tetrahedron
journal, February 2018
- Zhang, Liang; Lu, Cheng; Tieu, Kiet
- Scripta Materialia, Vol. 144
Vacancy loss at grain boundaries in quenched polycrystalline gold
journal, March 1980
- Siegel, R. W.; Chang, S. M.; Balluffi, R. W.
- Acta Metallurgica, Vol. 28, Issue 3
Works referencing / citing this record:
In situ TEM investigation of self-ion irradiation of nanoporous gold
journal, January 2019
- Briot, Nicolas J.; Kosmidou, Maria; Dingreville, Rémi
- Journal of Materials Science, Vol. 54, Issue 9
Effect of carbon nanotube on radiation resistance of CNT-Cu nanocomposite: MD simulation
journal, December 2019
- Hosseini, A.; Nasrabadi, M. N.; Esfandiarpour, A.
- Journal of Materials Science, Vol. 55, Issue 10
Interplay Between Grain Boundaries and Radiation Damage
journal, March 2019
- Barr, Christopher M.; El-Atwani, Osman; Kaoumi, Djamel
- JOM, Vol. 71, Issue 4
Listening to Radiation Damage In Situ: Passive and Active Acoustic Techniques
journal, November 2019
- Dennett, Cody A.; Choens, R. Charles; Taylor, Caitlin A.
- JOM, Vol. 72, Issue 1
Defect‐fluorite Gd 2 Zr 2 O 7 ceramics under helium irradiation: Amorphization, cell volume expansion, and multi‐stage bubble formation
journal, February 2019
- Huang, Zhangyi; Ma, Nannan; Qi, Jianqi
- Journal of the American Ceramic Society, Vol. 102, Issue 8