Unconventional Fermi surface in an insulating state
Abstract
Insulators occur in more than one guise; a recent finding was a class of topological insulators, which host a conducting surface juxtaposed with an insulating bulk. Here, we report the observation of an unusual insulating state with an electrically insulating bulk that simultaneously yields bulk quantum oscillations with characteristics of an unconventional Fermi liquid. We present quantum oscillation measurements of magnetic torque in high-purity single crystals of the Kondo insulator SmB6, which reveal quantum oscillation frequencies characteristic of a large three-dimensional conduction electron Fermi surface similar to the metallic rare earth hexaborides such as PrB6 and LaB6. As a result, the quantum oscillation amplitude strongly increases at low temperatures, appearing strikingly at variance with conventional metallic behavior.
- Authors:
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1355814
- Alternate Identifier(s):
- OSTI ID: 1186042
- Report Number(s):
- LA-UR-15-24709
Journal ID: ISSN 0036-8075
- Grant/Contract Number:
- SC0002613; AC52-06NA25396
- Resource Type:
- Published Article
- Journal Name:
- Science
- Additional Journal Information:
- Journal Name: Science Journal Volume: 349 Journal Issue: 6245; Journal ID: ISSN 0036-8075
- Publisher:
- American Association for the Advancement of Science (AAAS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; High Magnetic Field Science
Citation Formats
Tan, B. S., Hsu, Y. -. T., Zeng, B., Hatnean, M. C., Harrison, N., Zhu, Z., Hartstein, M., Kiourlappou, M., Srivastava, A., Johannes, M. D., Murphy, T. P., Park, J. -. H., Balicas, L., Lonzarich, G. G., Balakrishnan, G., and Sebastian, S. E. Unconventional Fermi surface in an insulating state. United States: N. p., 2015.
Web. doi:10.1126/science.aaa7974.
Tan, B. S., Hsu, Y. -. T., Zeng, B., Hatnean, M. C., Harrison, N., Zhu, Z., Hartstein, M., Kiourlappou, M., Srivastava, A., Johannes, M. D., Murphy, T. P., Park, J. -. H., Balicas, L., Lonzarich, G. G., Balakrishnan, G., & Sebastian, S. E. Unconventional Fermi surface in an insulating state. United States. https://doi.org/10.1126/science.aaa7974
Tan, B. S., Hsu, Y. -. T., Zeng, B., Hatnean, M. C., Harrison, N., Zhu, Z., Hartstein, M., Kiourlappou, M., Srivastava, A., Johannes, M. D., Murphy, T. P., Park, J. -. H., Balicas, L., Lonzarich, G. G., Balakrishnan, G., and Sebastian, S. E. Thu .
"Unconventional Fermi surface in an insulating state". United States. https://doi.org/10.1126/science.aaa7974.
@article{osti_1355814,
title = {Unconventional Fermi surface in an insulating state},
author = {Tan, B. S. and Hsu, Y. -. T. and Zeng, B. and Hatnean, M. C. and Harrison, N. and Zhu, Z. and Hartstein, M. and Kiourlappou, M. and Srivastava, A. and Johannes, M. D. and Murphy, T. P. and Park, J. -. H. and Balicas, L. and Lonzarich, G. G. and Balakrishnan, G. and Sebastian, S. E.},
abstractNote = {Insulators occur in more than one guise; a recent finding was a class of topological insulators, which host a conducting surface juxtaposed with an insulating bulk. Here, we report the observation of an unusual insulating state with an electrically insulating bulk that simultaneously yields bulk quantum oscillations with characteristics of an unconventional Fermi liquid. We present quantum oscillation measurements of magnetic torque in high-purity single crystals of the Kondo insulator SmB6, which reveal quantum oscillation frequencies characteristic of a large three-dimensional conduction electron Fermi surface similar to the metallic rare earth hexaborides such as PrB6 and LaB6. As a result, the quantum oscillation amplitude strongly increases at low temperatures, appearing strikingly at variance with conventional metallic behavior.},
doi = {10.1126/science.aaa7974},
journal = {Science},
number = 6245,
volume = 349,
place = {United States},
year = {Thu Jul 02 00:00:00 EDT 2015},
month = {Thu Jul 02 00:00:00 EDT 2015}
}
https://doi.org/10.1126/science.aaa7974
Web of Science
Figures / Tables:
Works referenced in this record:
Generalized Gradient Approximation Made Simple
journal, October 1996
- Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
- Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
Topological Kondo Insulators
journal, March 2010
- Dzero, Maxim; Sun, Kai; Galitski, Victor
- Physical Review Letters, Vol. 104, Issue 10
Temperature dependence of Sm valence in SmB 6 studied by X-ray absorption spectroscopy
journal, June 2009
- Mizumaki, Masaichiro; Tsutsui, Satoshi; Iga, Fumitoshi
- Journal of Physics: Conference Series, Vol. 176
Hall-effect evolution across a heavy-fermion quantum critical point
journal, December 2004
- Paschen, S.; Lühmann, T.; Wirth, S.
- Nature, Vol. 432, Issue 7019
Valence and magnetic ordering in intermediate valence compounds: TmSe versus SmB 6
journal, January 2006
- Derr, J.; Knebel, G.; Lapertot, G.
- Journal of Physics: Condensed Matter, Vol. 18, Issue 6
A Drastic Change of the Fermi Surface at a Critical Pressure in CeRhIn 5 : dHvA Study under Pressure
journal, April 2005
- Shishido, Hiroaki; Settai, Rikio; Harima, Hisatomo
- Journal of the Physical Society of Japan, Vol. 74, Issue 4
Two-dimensional Fermi surfaces in Kondo insulator SmB 6
journal, December 2014
- Li, G.; Xiang, Z.; Yu, F.
- Science, Vol. 346, Issue 6214
Sm : Kondo Insulator or Exotic Metal?
journal, February 1995
- Cooley, J. C.; Aronson, M. C.; Fisk, Z.
- Physical Review Letters, Vol. 74, Issue 9
Pressure-Induced Superconductivity in Quasi-2D
journal, May 2000
- Hegger, H.; Petrovic, C.; Moshopoulou, E. G.
- Physical Review Letters, Vol. 84, Issue 21
de Haas-van Alphen oscillations in superconducting states as a probe of gap anisotropy
journal, May 1993
- Miyake, K.
- Physica B: Condensed Matter, Vol. 186-188
String Theory, Quantum Phase Transitions, and the Emergent Fermi Liquid
journal, June 2009
- Čubrović, Mihailo; Zaanen, Jan; Schalm, Koenraad
- Science, Vol. 325, Issue 5939
Non-Fermi-liquid behavior in a heavy-fermion alloy at a magnetic instability
journal, May 1994
- Löhneysen, H. v.; Pietrus, T.; Portisch, G.
- Physical Review Letters, Vol. 72, Issue 20
Generalized Lifshitz-Kosevich scaling at quantum criticality from the holographic correspondence
journal, April 2010
- Hartnoll, Sean A.; Hofman, Diego M.
- Physical Review B, Vol. 81, Issue 15
Magnetic excitations in SmB6 single crystals
journal, May 1993
- Alekseev, P. A.; Mignot, J. -M.; Rossat-Mignod, J.
- Physica B: Condensed Matter, Vol. 186-188
de Haas van Alphen effect in heavy fermion compounds—effective mass and non-Fermi-liquid behaviour
journal, April 2008
- McCollam, A.; Xia, J. -S.; Flouquet, J.
- Physica B: Condensed Matter, Vol. 403, Issue 5-9
LaB6 and SmB6 (001) surfaces studied by angle-resolved XPS, LEED and ISS
journal, July 1979
- Aono, M.; Nishitani, R.; Oshima, C.
- Surface Science, Vol. 86
From unconventional insulating behavior towards conventional magnetism in the intermediate-valence compound
journal, May 2008
- Derr, J.; Knebel, G.; Braithwaite, D.
- Physical Review B, Vol. 77, Issue 19
Magnetically mediated superconductivity in heavy fermion compounds
journal, July 1998
- Mathur, N. D.; Grosche, F. M.; Julian, S. R.
- Nature, Vol. 394, Issue 6688
Heavy-fermion quasiparticles in
journal, April 1988
- Taillefer, L.; Lonzarich, G. G.
- Physical Review Letters, Vol. 60, Issue 15
Disorder-Sensitive Phase Formation Linked to Metamagnetic Quantum Criticality
journal, November 2004
- Grigera, S. A.
- Science, Vol. 306, Issue 5699
Quantum Criticality Without Tuning in the Mixed Valence Compound -YbAlB4
journal, January 2011
- Matsumoto, Y.; Nakatsuji, S.; Kuga, K.
- Science, Vol. 331, Issue 6015
Are Kondo insulators gapless?
journal, May 1993
- Coleman, P.; Miranda, E.; Tsvelik, A.
- Physica B: Condensed Matter, Vol. 186-188
High-Pressure Ground State of : Electronic Conduction and Long Range Magnetic Order
journal, April 2005
- Barla, A.; Derr, J.; Sanchez, J. P.
- Physical Review Letters, Vol. 94, Issue 16
Influence of the electron-phonon interaction on the de Haas-van Alphen effect in mercury
journal, December 1980
- Elliott, M.; Ellis, T.; Springford, M.
- Journal of Physics F: Metal Physics, Vol. 10, Issue 12
Two-Dimensional Magnetotransport in the Extreme Quantum Limit
journal, May 1982
- Tsui, D. C.; Stormer, H. L.; Gossard, A. C.
- Physical Review Letters, Vol. 48, Issue 22
Quantum phase transitions in heavy fermion metals and Kondo insulators
journal, March 2013
- Si, Qimiao; Paschen, Silke
- physica status solidi (b), Vol. 250, Issue 3
Singular or non-Fermi liquids
journal, May 2002
- Varma, C. M.; Nussinov, Z.; van Saarloos, Wim
- Physics Reports, Vol. 361, Issue 5-6
Anomalous Quantum Hall Effect: An Incompressible Quantum Fluid with Fractionally Charged Excitations
journal, May 1983
- Laughlin, R. B.
- Physical Review Letters, Vol. 50, Issue 18
Non-Fermi-liquid nature of the normal state of itinerant-electron ferromagnets
journal, November 2001
- Pfleiderer, C.; Julian, S. R.; Lonzarich, G. G.
- Nature, Vol. 414, Issue 6862
Low-temperature magnetic fluctuations in the Kondo insulator
journal, April 2014
- Biswas, P. K.; Salman, Z.; Neupert, T.
- Physical Review B, Vol. 89, Issue 16
Gap state of SmB6
journal, May 1993
- Nanba, T.; Ohta, H.; Motokawa, M.
- Physica B: Condensed Matter, Vol. 186-188
De Haas-van Alphen effect in rare-earth hexaborides (RE=Pr, Nd, Gd)
journal, October 1991
- Behler, S.; Winzer, K.
- Zeitschrift f�r Physik B Condensed Matter, Vol. 82, Issue 3
Large, high quality single-crystals of the new Topological Kondo Insulator, SmB6
journal, October 2013
- Hatnean, M. Ciomaga; Lees, M. R.; Paul, D. McK.
- Scientific Reports, Vol. 3, Issue 1
Influence of Electron-Phonon Interactions on the de Haas-van Alphen Effect
journal, September 1970
- Engelsberg, S.; Simpson, G.
- Physical Review B, Vol. 2, Issue 6
Magnetic and Semiconducting Properties of Sm
journal, February 1969
- Menth, A.; Buehler, E.; Geballe, T. H.
- Physical Review Letters, Vol. 22, Issue 7
Specific heat of SmB6 at very low temperatures
journal, May 2006
- Flachbart, K.; Gabáni, S.; Neumaier, K.
- Physica B: Condensed Matter, Vol. 378-380
Rare-earth compounds with mixed valencies
journal, August 1974
- Mott, N. F.
- Philosophical Magazine, Vol. 30, Issue 2
de Haas-van Alphen Effect in the Heavy-Electron Compound Ce
journal, September 1986
- Reinders, P. H. P.; Springford, M.; Coleridge, P. T.
- Physical Review Letters, Vol. 57, Issue 13
Light scattering from gap excitations and bound states in
journal, November 1995
- Nyhus, P.; Cooper, S. L.; Fisk, Z.
- Physical Review B, Vol. 52, Issue 20
Fermi Surface and Cyclotron Mass of CeB 6
journal, October 1989
- Ōnuki, Yoshichika; Komatsubara, Takemi; H. P. Reinders, Paul
- Journal of the Physical Society of Japan, Vol. 58, Issue 10
Electronic and Magnetic Structure of Sm
journal, February 1970
- Cohen, R. L.; Eibschütz, M.; West, K. W.
- Physical Review Letters, Vol. 24, Issue 8
Destruction of the gap in the intermediate valence compound SmB6 by neutron irradiation
journal, October 1983
- Morillo, Joseph; de Novion, Charles-Henri; Jun, Jan
- Solid State Communications, Vol. 48, Issue 4
Hall Mobility and Optical Conductivity in SmB 6
journal, February 1994
- Kasuya, Tadao
- Journal of the Physical Society of Japan, Vol. 63, Issue 2
Towards resolution of the Fermi surface in underdoped high- T c superconductors
journal, September 2012
- Sebastian, Suchitra E.; Harrison, Neil; Lonzarich, Gilbert G.
- Reports on Progress in Physics, Vol. 75, Issue 10
Specific heat of Nd Ca B single crystals
journal, March 2011
- Stankiewicz, Jolanta; Evangelisti, Marco; Fisk, Zachary
- Physical Review B, Vol. 83, Issue 11
Magnetic Field-Induced Superconductivity in the Ferromagnet URhGe
journal, August 2005
- Levy, F.
- Science, Vol. 309, Issue 5739