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Title: Atomic moments in Mn2CoAl thin films analyzed by X-ray magnetic circular dichroism

Abstract

Spin gapless semiconductors are known to be strongly affected by structural disorder when grown epitaxially as thin films. The magnetic properties of Mn2CoAl thin films grown on GaAs (001) substrates are investigated here as a function of annealing. This study investigates the atomic-specific magnetic moments of Mn and Co atoms measured through X-ray magnetic circular dichroism as a function of annealing and the consequent structural ordering. Results indicate that the structural distortion mainly affects the Mn atoms as seen by the reduction of the magnetic moment from its predicted value.

Authors:
 [1];  [1];  [2];  [2];  [1]
  1. Northeastern Univ., Boston, MA (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
Publication Date:
Research Org.:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1174115
Report Number(s):
BNL-107537-2015-JA
Journal ID: ISSN 0021-8979; JAPIAU; TRN: US1500487
Grant/Contract Number:  
SC00112704
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Applied Physics
Additional Journal Information:
Journal Volume: 116; Journal Issue: 21; Journal ID: ISSN 0021-8979
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; magnetic moments; magnetic annealing; coal; magnetic films; thin film growth

Citation Formats

Jamer, M. E., Assaf, B. A., Sterbinsky, G. E., Arena, D. A., and Heiman, D. Atomic moments in Mn2CoAl thin films analyzed by X-ray magnetic circular dichroism. United States: N. p., 2014. Web. doi:10.1063/1.4903771.
Jamer, M. E., Assaf, B. A., Sterbinsky, G. E., Arena, D. A., & Heiman, D. Atomic moments in Mn2CoAl thin films analyzed by X-ray magnetic circular dichroism. United States. https://doi.org/10.1063/1.4903771
Jamer, M. E., Assaf, B. A., Sterbinsky, G. E., Arena, D. A., and Heiman, D. Fri . "Atomic moments in Mn2CoAl thin films analyzed by X-ray magnetic circular dichroism". United States. https://doi.org/10.1063/1.4903771. https://www.osti.gov/servlets/purl/1174115.
@article{osti_1174115,
title = {Atomic moments in Mn2CoAl thin films analyzed by X-ray magnetic circular dichroism},
author = {Jamer, M. E. and Assaf, B. A. and Sterbinsky, G. E. and Arena, D. A. and Heiman, D.},
abstractNote = {Spin gapless semiconductors are known to be strongly affected by structural disorder when grown epitaxially as thin films. The magnetic properties of Mn2CoAl thin films grown on GaAs (001) substrates are investigated here as a function of annealing. This study investigates the atomic-specific magnetic moments of Mn and Co atoms measured through X-ray magnetic circular dichroism as a function of annealing and the consequent structural ordering. Results indicate that the structural distortion mainly affects the Mn atoms as seen by the reduction of the magnetic moment from its predicted value.},
doi = {10.1063/1.4903771},
journal = {Journal of Applied Physics},
number = 21,
volume = 116,
place = {United States},
year = {Fri Dec 05 00:00:00 EST 2014},
month = {Fri Dec 05 00:00:00 EST 2014}
}

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Works referenced in this record:

Proposal for a New Class of Materials: Spin Gapless Semiconductors
journal, April 2008


Search for spin gapless semiconductors: The case of inverse Heusler compounds
journal, January 2013

  • Skaftouros, S.; Özdoğan, K.; Şaşıoğlu, E.
  • Applied Physics Letters, Vol. 102, Issue 2
  • DOI: 10.1063/1.4775599

Realization of Spin Gapless Semiconductors: The Heusler Compound Mn 2 CoAl
journal, March 2013


The zero-magnetization Heusler ferrimagnet
journal, May 2013

  • Hakimi, M.; Venkatesan, M.; Rode, K.
  • Journal of Applied Physics, Vol. 113, Issue 17
  • DOI: 10.1063/1.4794744

Magnetic and transport properties of Mn 2 CoAl oriented films
journal, September 2013

  • Jamer, Michelle E.; Assaf, Badih A.; Devakul, Trithep
  • Applied Physics Letters, Vol. 103, Issue 14
  • DOI: 10.1063/1.4823601

Magneto-transport properties of oriented Mn 2 CoAl films sputtered on thermally oxidized Si substrates
journal, June 2014

  • Xu, G. Z.; Du, Y.; Zhang, X. M.
  • Applied Physics Letters, Vol. 104, Issue 24
  • DOI: 10.1063/1.4884203

Anomalous Hall effect in stoichiometric Heusler alloys with native disorder: A first-principles study
journal, July 2013


Conditions for spin-gapless semiconducting behavior in Mn 2 CoAl inverse Heusler compound
journal, March 2014

  • Galanakis, I.; Özdoğan, K.; Şaşıoğlu, E.
  • Journal of Applied Physics, Vol. 115, Issue 9
  • DOI: 10.1063/1.4867917

Electronic structure and magnetism of Fe 3 x V x X ( X = Si , Ga, and Al) alloys by the KKR-CPA method
journal, November 1999


Anomalous magnetic properties and Hall effect in ferromagnetic Co2MnAl epilayers
journal, May 2004

  • Chen, Y. J.; Basiaga, D.; O’Brien, J. R.
  • Applied Physics Letters, Vol. 84, Issue 21
  • DOI: 10.1063/1.1755842

X-ray circular dichroism as a probe of orbital magnetization
journal, March 1992


X-ray circular dichroism and local magnetic fields
journal, February 1993


ATHENA , ARTEMIS , HEPHAESTUS : data analysis for X-ray absorption spectroscopy using IFEFFIT
journal, June 2005


Accuracy of the spin sum rule in XMCD for the transition-metal L edges from manganese to copper
journal, November 2009


Localized Magnetic Moments and Pauling Valence in Manganese Metal, Some 3d-Transition Alloys and Intermetallic Compounds
journal, July 1968

  • Môri, Nobuo; Mitsui, Tadayasu
  • Journal of the Physical Society of Japan, Vol. 25, Issue 1
  • DOI: 10.1143/JPSJ.25.82

The CTM4XAS program for EELS and XAS spectral shape analysis of transition metal L edges
journal, October 2010


Phase stability of chromium based compensated ferrimagnets with inverse Heusler structure
journal, September 2013


Multiple phases in sputtered Cr2CoGa films
journal, June 2014


Works referencing / citing this record:

Theory of Heusler and Full-Heusler Compounds
book, November 2015


Spin-filter and spin-gapless semiconductors: The case of Heusler compounds
journal, May 2016

  • Galanakis, I.; Özdoğan, K.; Şaşıoğlu, E.
  • AIP Advances, Vol. 6, Issue 5
  • DOI: 10.1063/1.4943761

Exploring disorder in the spin gapless semiconductor Mn 2 CoAl
journal, September 2019

  • Buckley, Robert G.; Butler, Tane; Pot, Catherine
  • Materials Research Express, Vol. 6, Issue 10
  • DOI: 10.1088/2053-1591/ab3bd3

Exploring Disorder in the Spin Gapless Semiconductor Mn$_2$CoAl
text, January 2019