Magnetic inhomogeneity in a multiferroic EuTiO3 thin film

Geng, Yanan; Lee, J. H.; Schlom, D. G.; Freeland, J. W.; Wu, Weida

doi:10.1103/PhysRevB.87.121109

Title: Magnetic inhomogeneity in a multiferroic EuTiO₃ thin film

Authors:: Geng, Yanan; Lee, J. H.; Schlom, D. G.; Freeland, J. W.; Wu, Weida

Publication Date:: Mon Mar 18 00:00:00 EDT 2013

Sponsoring Org.:: USDOE

OSTI Identifier:: 1103916

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Physical Review. B, Condensed Matter and Materials Physics

Additional Journal Information:: Journal Name: Physical Review. B, Condensed Matter and Materials Physics Journal Volume: 87 Journal Issue: 12; Journal ID: ISSN 1098-0121

Publisher:: American Physical Society

Country of Publication:: United States

Language:: English

Citation Formats


                    Geng, Yanan, Lee, J. H., Schlom, D. G., Freeland, J. W., and Wu, Weida. Magnetic inhomogeneity in a multiferroic EuTiO3 thin film.  United States: N. p., 2013. 
Web.  doi:10.1103/PhysRevB.87.121109.

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                    Geng, Yanan, Lee, J. H., Schlom, D. G., Freeland, J. W., & Wu, Weida. Magnetic inhomogeneity in a multiferroic EuTiO3 thin film.  United States.  https://doi.org/10.1103/PhysRevB.87.121109

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                    Geng, Yanan, Lee, J. H., Schlom, D. G., Freeland, J. W., and Wu, Weida. Mon .  
"Magnetic inhomogeneity in a multiferroic EuTiO3 thin film".  United States.  https://doi.org/10.1103/PhysRevB.87.121109.

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@article{osti_1103916,

  title        = {Magnetic inhomogeneity in a multiferroic EuTiO3 thin film},

  author       = {Geng, Yanan and Lee, J. H. and Schlom, D. G. and Freeland, J. W. and Wu, Weida},

  abstractNote = {},

  doi          = {10.1103/PhysRevB.87.121109},

  journal      = {Physical Review. B, Condensed Matter and Materials Physics},

  number       = 12,

  volume       = 87,

  place        = {United States},

  year         = {Mon Mar 18 00:00:00 EDT 2013},

  month        = {Mon Mar 18 00:00:00 EDT 2013}

}

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Works referenced in this record:

MATERIALS SCIENCE: The Renaissance of Magnetoelectric Multiferroics
journal, July 2005

Spaldin, N. A.
Science, Vol. 309, Issue 5733
DOI: 10.1126/science.1113357

First-principles prediction of oxygen octahedral rotations in perovskite-structure EuTiO $_{3}$
journal, March 2012

Rushchanskii, Konstantin Z.; Spaldin, Nicola A.; Ležaić, Marjana
Physical Review B, Vol. 85, Issue 10
DOI: 10.1103/PhysRevB.85.104109

Electronically soft phases in manganites
journal, February 2005

Milward, G. C.; Calderón, M. J.; Littlewood, P. B.
Nature, Vol. 433, Issue 7026
DOI: 10.1038/nature03300

Room-temperature ferroelectricity in strained SrTiO₃
journal, August 2004

Haeni, J. H.; Irvin, P.; Chang, W.
Nature, Vol. 430, Issue 7001, p. 758-761
DOI: 10.1038/nature02773

A Thin Film Approach to Engineering Functionality into Oxides
journal, August 2008

Schlom, Darrell G.; Chen, Long-Qing; Pan, Xiaoqing
Journal of the American Ceramic Society, Vol. 91, Issue 8
DOI: 10.1111/j.1551-2916.2008.02556.x

Reversible control of magnetic interactions by electric field in a single-phase material
journal, January 2013

Ryan, P. J.; Kim, J-W; Birol, T.
Nature Communications, Vol. 4, Issue 1
DOI: 10.1038/ncomms2329

Contribution of Eu 4f states to the magnetic anisotropy of EuO
journal, April 2009

Arenholz, E.; Schmehl, A.; Schlom, D. G.
Journal of Applied Physics, Vol. 105, Issue 7
DOI: 10.1063/1.3054364

Low temperature magnetism in the perovskite substrate DyScO3
journal, April 2009

Ke, X.; Adamo, C.; Schlom, D. G.
Applied Physics Letters, Vol. 94, Issue 15
DOI: 10.1063/1.3117190

Why Are There so Few Magnetic Ferroelectrics?
journal, July 2000

Hill, Nicola A.
The Journal of Physical Chemistry B, Vol. 104, Issue 29
DOI: 10.1021/jp000114x

Thermal expansion of the new perovskite substrates DyScO ₃ and GdScO ₃
journal, April 2005

Biegalski, M. D.; Haeni, J. H.; Trolier-McKinstry, S.
Journal of Materials Research, Vol. 20, Issue 4
DOI: 10.1557/JMR.2005.0126

The magnetoelectric effect in transition metal oxides: Insights and the rational design of new materials from first principles
journal, October 2012

Birol, Turan; Benedek, Nicole A.; Das, Hena
Current Opinion in Solid State and Materials Science, Vol. 16, Issue 5
DOI: 10.1016/j.cossms.2012.08.002

A strong ferroelectric ferromagnet created by means of spin–lattice coupling
journal, August 2010

Lee, June Hyuk; Fang, Lei; Vlahos, Eftihia
Nature, Vol. 466, Issue 7309
DOI: 10.1038/nature09331

Coupling between magnetism and dielectric properties in quantum paraelectric ${EuTiO}_{3}$
journal, July 2001

Katsufuji, T.; Takagi, H.
Physical Review B, Vol. 64, Issue 5
DOI: 10.1103/PhysRevB.64.054415

Antiferrodistortive phase transition in EuTiO $_{3}$
journal, August 2012

Goian, V.; Kamba, S.; Pacherová, O.
Physical Review B, Vol. 86, Issue 5
DOI: 10.1103/PhysRevB.86.054112

Crystal chemistry of GdScO3, DyScO3, SmScO3 and NdScO3
journal, January 2007

Veličkov, Boža; Kahlenberg, Volker; Bertram, Rainer
Zeitschrift für Kristallographie, Vol. 222, Issue 9
DOI: 10.1524/zkri.2007.222.9.466

EuTiO $_{3}$ magnetic structure studied by neutron powder diffraction and resonant x-ray scattering
journal, September 2012

Scagnoli, Valerio; Allieta, Mattia; Walker, Helen
Physical Review B, Vol. 86, Issue 9
DOI: 10.1103/PhysRevB.86.094432

Frequency modulation detection using high‐ Q cantilevers for enhanced force microscope sensitivity
journal, January 1991

Albrecht, T. R.; Grütter, P.; Horne, D.
Journal of Applied Physics, Vol. 69, Issue 2
DOI: 10.1063/1.347347

Magnetic imaging of a supercooling glass transition in a weakly disordered ferromagnet
journal, October 2006

Wu, Weida; Israel, Casey; Hur, Namjung
Nature Materials, Vol. 5, Issue 11
DOI: 10.1038/nmat1743

Emergent Superstructural Dynamic Order due to Competing Antiferroelectric and Antiferrodistortive Instabilities in Bulk ${EuTiO}_{3}$
journal, January 2013

Kim, Jong-Woo; Thompson, Paul; Brown, Simon
Physical Review Letters, Vol. 110, Issue 2
DOI: 10.1103/PhysRevLett.110.027201

Magnetic and Electric Phase Control in Epitaxial ${EuTiO}_{3}$ from First Principles
journal, December 2006

Fennie, Craig J.; Rabe, Karin M.
Physical Review Letters, Vol. 97, Issue 26
DOI: 10.1103/PhysRevLett.97.267602

Microscopic evidence of a strain-enhanced ferromagnetic state in LaCoO3 thin films
journal, August 2009

Park, S.; Ryan, P.; Karapetrova, E.
Applied Physics Letters, Vol. 95, Issue 7
DOI: 10.1063/1.3206667

Understanding and Revisiting Properties of ${EuTiO}_{3}$ Bulk Material and Films from First Principles
journal, December 2012

Yang, Yurong; Ren, Wei; Wang, Dawei
Physical Review Letters, Vol. 109, Issue 26
DOI: 10.1103/PhysRevLett.109.267602

Multiferroics progress and prospects in thin films
journal, January 2007

Ramesh, R.; Spaldin, Nicola A.
Nature Materials, Vol. 6, Issue 1, p. 21-29
DOI: 10.1038/nmat1805

Multiferroics: a magnetic twist for ferroelectricity
journal, January 2007

Cheong, Sang-Wook; Mostovoy, Maxim
Nature Materials, Vol. 6, Issue 1
DOI: 10.1038/nmat1804

Enhancement of Ferroelectricity in Strained BaTiO₃ Thin Films
journal, November 2004

Choi, K. J.; Biegalski, M.; Li, Y. L.
Science, Vol. 306, Issue 5698, p. 1005-1009
DOI: 10.1126/science.1103218

Pancakelike Ising domains and charge-ordered superlattice domains in ${LuFe}_{2} O_{4}$
journal, May 2009

Park, S.; Horibe, Y.; Choi, Y. J.
Physical Review B, Vol. 79, Issue 18
DOI: 10.1103/PhysRevB.79.180401

Multiferroics and magnetoelectrics: thin films and nanostructures
journal, October 2008

Martin, L. W.; Crane, S. P.; Chu, Y-H
Journal of Physics: Condensed Matter, Vol. 20, Issue 43
DOI: 10.1088/0953-8984/20/43/434220

Role of intrinsic disorder in the structural phase transition of magnetoelectric EuTiO $_{3}$
journal, May 2012

Allieta, Mattia; Scavini, Marco; Spalek, Leszek J.
Physical Review B, Vol. 85, Issue 18
DOI: 10.1103/PhysRevB.85.184107

Magnetic force microscopy: General principles and application to longitudinal recording media
journal, August 1990

Rugar, D.; Mamin, H. J.; Guethner, P.
Journal of Applied Physics, Vol. 68, Issue 3
DOI: 10.1063/1.346713

Multiferroic and magnetoelectric materials
journal, August 2006

Eerenstein, W.; Mathur, N. D.; Scott, J. F.
Nature, Vol. 442, Issue 7104
DOI: 10.1038/nature05023

Strain Tuning of Ferroelectric Thin Films
journal, August 2007

Schlom, Darrell G.; Chen, Long-Qing; Eom, Chang-Beom
Annual Review of Materials Research, Vol. 37, Issue 1
DOI: 10.1146/annurev.matsci.37.061206.113016

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Title: Magnetic inhomogeneity in a multiferroic EuTiO3 thin film

Citation Formats

MATERIALS SCIENCE: The Renaissance of Magnetoelectric Multiferroics journal, July 2005

First-principles prediction of oxygen octahedral rotations in perovskite-structure EuTiO 3 journal, March 2012

Electronically soft phases in manganites journal, February 2005

Room-temperature ferroelectricity in strained SrTiO3 journal, August 2004

A Thin Film Approach to Engineering Functionality into Oxides journal, August 2008

Reversible control of magnetic interactions by electric field in a single-phase material journal, January 2013

Contribution of Eu 4f states to the magnetic anisotropy of EuO journal, April 2009

Low temperature magnetism in the perovskite substrate DyScO3 journal, April 2009

Why Are There so Few Magnetic Ferroelectrics? journal, July 2000

Thermal expansion of the new perovskite substrates DyScO 3 and GdScO 3 journal, April 2005

The magnetoelectric effect in transition metal oxides: Insights and the rational design of new materials from first principles journal, October 2012

A strong ferroelectric ferromagnet created by means of spin–lattice coupling journal, August 2010

Coupling between magnetism and dielectric properties in quantum paraelectric EuTiO 3 journal, July 2001

Antiferrodistortive phase transition in EuTiO 3 journal, August 2012

Crystal chemistry of GdScO3, DyScO3, SmScO3 and NdScO3 journal, January 2007

EuTiO 3 magnetic structure studied by neutron powder diffraction and resonant x-ray scattering journal, September 2012

Frequency modulation detection using high‐ Q cantilevers for enhanced force microscope sensitivity journal, January 1991

Magnetic imaging of a supercooling glass transition in a weakly disordered ferromagnet journal, October 2006

Emergent Superstructural Dynamic Order due to Competing Antiferroelectric and Antiferrodistortive Instabilities in Bulk EuTiO 3 journal, January 2013

Magnetic and Electric Phase Control in Epitaxial EuTiO 3 from First Principles journal, December 2006

Microscopic evidence of a strain-enhanced ferromagnetic state in LaCoO3 thin films journal, August 2009

Understanding and Revisiting Properties of EuTiO 3 Bulk Material and Films from First Principles journal, December 2012

Multiferroics progress and prospects in thin films journal, January 2007

Multiferroics: a magnetic twist for ferroelectricity journal, January 2007

Enhancement of Ferroelectricity in Strained BaTiO3 Thin Films journal, November 2004

Pancakelike Ising domains and charge-ordered superlattice domains in LuFe 2 O 4 journal, May 2009

Multiferroics and magnetoelectrics: thin films and nanostructures journal, October 2008

Role of intrinsic disorder in the structural phase transition of magnetoelectric EuTiO 3 journal, May 2012

Magnetic force microscopy: General principles and application to longitudinal recording media journal, August 1990

Multiferroic and magnetoelectric materials journal, August 2006

Strain Tuning of Ferroelectric Thin Films journal, August 2007

Title: Magnetic inhomogeneity in a multiferroic EuTiO₃ thin film

MATERIALS SCIENCE: The Renaissance of Magnetoelectric Multiferroics
journal, July 2005

First-principles prediction of oxygen octahedral rotations in perovskite-structure EuTiO $_{3}$
journal, March 2012

Electronically soft phases in manganites
journal, February 2005

Room-temperature ferroelectricity in strained SrTiO₃
journal, August 2004

A Thin Film Approach to Engineering Functionality into Oxides
journal, August 2008

Reversible control of magnetic interactions by electric field in a single-phase material
journal, January 2013

Contribution of Eu 4f states to the magnetic anisotropy of EuO
journal, April 2009

Low temperature magnetism in the perovskite substrate DyScO3
journal, April 2009

Why Are There so Few Magnetic Ferroelectrics?
journal, July 2000

Thermal expansion of the new perovskite substrates DyScO ₃ and GdScO ₃
journal, April 2005

The magnetoelectric effect in transition metal oxides: Insights and the rational design of new materials from first principles
journal, October 2012

A strong ferroelectric ferromagnet created by means of spin–lattice coupling
journal, August 2010

Coupling between magnetism and dielectric properties in quantum paraelectric ${EuTiO}_{3}$
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Antiferrodistortive phase transition in EuTiO $_{3}$
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Crystal chemistry of GdScO3, DyScO3, SmScO3 and NdScO3
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EuTiO $_{3}$ magnetic structure studied by neutron powder diffraction and resonant x-ray scattering
journal, September 2012

Frequency modulation detection using high‐ Q cantilevers for enhanced force microscope sensitivity
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Magnetic imaging of a supercooling glass transition in a weakly disordered ferromagnet
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Emergent Superstructural Dynamic Order due to Competing Antiferroelectric and Antiferrodistortive Instabilities in Bulk ${EuTiO}_{3}$
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Magnetic and Electric Phase Control in Epitaxial ${EuTiO}_{3}$ from First Principles
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