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Three-dimensional ferroelectric domain imaging of epitaxial BiFeO{sub } thin films using angle-resolved piezoresponse force microscopy.

Journal Article · · Appl. Phys. Lett.
DOI:https://doi.org/10.1063/1.3487933· OSTI ID:992403

Here we introduce angle-resolved piezoresponse force microscopy (AR-PFM), whereby the sample is rotated by 30{sup o} increments around the surface normal vector and the in-plane PFM phase signals are collected at each angle. We obtained the AR-PFM images of BaTiO{sub 3} single crystal and cube-on-cube epitaxial (001) BiFeO{sub 3} (BFO) thin film on SrRuO{sub 3}/SrTiO{sub 3} substrate, and confirmed that the AR-PFM provides more unambiguous information on the in-plane polarization directions than the conventional PFM method. Moreover, we found eight additional in-plane polarization variants in epitaxial BFO thin films, which are formed to mitigate highly unstable charged domain boundaries.

Research Organization:
Argonne National Laboratory (ANL)
Sponsoring Organization:
SC
DOE Contract Number:
AC02-06CH11357
OSTI ID:
992403
Report Number(s):
ANL/MSD/JA-67858
Journal Information:
Appl. Phys. Lett., Journal Name: Appl. Phys. Lett. Journal Issue: 2010 Vol. 97; ISSN 0003-6951
Country of Publication:
United States
Language:
ENGLISH

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