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RAPID SEPARATION METHOD FOR ACTINIDES IN EMERGENCY AIR FILTER SAMPLES

Journal Article · · Applied Radiation and Isotopes

A new rapid method for the determination of actinides and strontium in air filter samples has been developed at the Savannah River Site Environmental Lab (Aiken, SC, USA) that can be used in emergency response situations. The actinides and strontium in air filter method utilizes a rapid acid digestion method and a streamlined column separation process with stacked TEVA, TRU and Sr Resin cartridges. Vacuum box technology and rapid flow rates are used to reduce analytical time. Alpha emitters are prepared using cerium fluoride microprecipitation for counting by alpha spectrometry. The purified {sup 90}Sr fractions are mounted directly on planchets and counted by gas flow proportional counting. The method showed high chemical recoveries and effective removal of interferences. This new procedure was applied to emergency air filter samples received in the NRIP Emergency Response exercise administered by the National Institute for Standards and Technology (NIST) in April, 2009. The actinide and {sup 90}Sr in air filter results were reported in {approx}4 hours with excellent quality.

Research Organization:
SRS
Sponsoring Organization:
DOE
DOE Contract Number:
AC09-08SR22470
OSTI ID:
972784
Report Number(s):
SRNS-STI-2010-00069
Journal Information:
Applied Radiation and Isotopes, Journal Name: Applied Radiation and Isotopes; ISSN 0969-8043; ISSN ARISEF
Country of Publication:
United States
Language:
English

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