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Method of making an icosahedral boride structure

Patent ·
OSTI ID:879999
 [1];  [2];  [3];  [4];  [5]
  1. 3712 Silver Ave. SE., Albuquerque, NM 87108
  2. 939 Buena Vista Dr., SE., Apt. F203, Albuquerque, NM 87106
  3. 4409 Buckingham Dr., El Paso, TX 79902
  4. 62 Avenida Del Sol, Cedar Crest, NM 87008
  5. 1502 Harvard Ct. NE., Albuquerque, NM 87106

A method for fabricating thin films of an icosahedral boride on a silicon carbide (SiC) substrate is provided. Preferably the icosahedral boride layer is comprised of either boron phosphide (B.sub.12 P.sub.2) or boron arsenide (B.sub.12 As.sub.2). The provided method achieves improved film crystallinity and lowered impurity concentrations. In one aspect, an epitaxially grown layer of B.sub.12 P.sub.2 with a base layer or substrate of SiC is provided. In another aspect, an epitaxially grown layer of B.sub.12 As.sub.2 with a base layer or substrate of SiC is provided. In yet another aspect, thin films of B.sub.12 P.sub.2 or B.sub.12 As.sub.2 are formed on SiC using CVD or other vapor deposition means. If CVD techniques are employed, preferably the deposition temperature is above 1050.degree. C., more preferably in the range of 1100.degree. C. to 1400.degree. C., and still more preferably approximately 1150.degree. C.

Research Organization:
Sandia Corporation
DOE Contract Number:
AC04-94AL85000
Assignee:
OSTI
Patent Number(s):
US 6,841,456
Application Number:
10/418018
OSTI ID:
879999
Country of Publication:
United States
Language:
English

References (12)

Preparation and Properties of Boron Arsenide Films journal January 1974
Hetero-Epitaxial Growth of Lower Boron Phosphide on Silicon Substrate Using PH 3 -B 2 H 6 -H 2 System journal October 1973
Crystals and Epitaxial Layers of Boron Phosphide journal January 1971
Epitaxial Growth of Rhombohedral Boron Phosphide Single Crystalline Films by Chemical Vapor Deposition journal October 1997
Struktur des borreichen Borphosphids journal November 1974
Defect clustering and self-healing of electron-irradiated boron-rich solids journal May 1995
Thermoelectric Properties of Boron and Boron Phosphide CVD Wafers journal October 1997
Double-Layer Epitaxial Growth of Si and B 13 P 2 on Si Substrates and Some Electrical Properties of Si Layers journal August 1974
Hetero-Epitaxial Growth of Lower Boron Arsenide on Si Substrate Using AsH 3 -B 2 H 6 -H 2 System journal December 1973
Chemical vapour deposition of boron subarsenide using halide reactants journal December 1986
New group III-group V compounds: BP and BAs journal April 1958
The Preparation and Properties of Boron Phosphides and Arsenides 1 journal March 1960

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