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Transition metal-free olefin polymerization catalyst

Patent ·
OSTI ID:874003

Ethylene and/or propylene are polymerized to form high molecular weight, linear polymers by contacting ethylene and/or propylene monomer, in the presence of an inert reaction medium, with a catalyst system which consists essentially of (1) an aluminum alkyl component, such as trimethylaluminum, triethylaluminum, triisobutylaluminum, tri-n-octylaluminum and diethylaluminum hydride and (2) a Lewis acid or Lewis acid derivative component, such as B (C.sub.6 F.sub.5).sub.3, [(CH.sub.3).sub.2 N (H) (C.sub.6 H.sub.5)].sup.+ [B (C.sub.6 F.sub.5)4].sup.-, [(C.sub.2 H.sub.5).sub.3 NH].sup.+ [B C.sub.6 F.sub.5).sub.4 ],.sup.-, [C(C.sub.6 F.sub.5).sub.3 ].sup.+ [B(C.sub.6 F.sub.5).sub.4 ].sup.-, (C.sub.2 H.sub.5).sub.2 Al(OCH.sub.3), (C.sub.2 H.sub.5).sub.2 Al(2,6-di-t-butyl-4-methylphenoxide), (C.sub.2 H.sub.5)Al(2,6 -di-t-butylphenoxide).sub.2, (C.sub.2 H.sub.5).sub.2 Al(2,6-di-t-butylphonoxide) , 2,6 -di-t-butylphenol.multidot.methylaluminoxane or an alkylaluminoxane, and which may be completely free any transition metal component(s).

Research Organization:
Pennsylvania State University, University Park, PA (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
FG02-84ER13295
Assignee:
Penn State Research Foundation (University Park, PA)
Patent Number(s):
6,291,387
Application Number:
09/273,128
OSTI ID:
874003
Country of Publication:
United States
Language:
English

References (12)

Preparation of “living” polypropylenes by a soluble vanadium-based Ziegler catalyst journal May 1979
High-molecular-weight polyethylene: growth reactions at bis(dichloroaluminium)ethane and trialkylaluminium journal June 1992
Chromocene catalysts for ethylene polymerization: Scope of the polymerization journal September 1972
Ziegler-Natta Catalysis book January 1980
New Pd(II)- and Ni(II)-Based Catalysts for Polymerization of Ethylene and .alpha.-Olefins journal June 1995
Cationic Aluminum Alkyl Complexes Incorporating Amidinate Ligands. Transition-Metal-Free Ethylene Polymerization Catalysts journal August 1997
Highly Active Iron and Cobalt Catalysts for the Polymerization of Ethylene journal April 1998
Cationic Aluminum Alkyl Complexes Incorporating Aminotroponiminate Ligands journal July 1998
Synthesis and Structures of Mono- and Bis(amidinate) Complexes of Aluminum journal November 1997
Aluminum Alkyl Complexes Containing Guanidinate Ligands journal July 1998
Aluminum Complexes Incorporating Bulky Nitrogen and Sulfur Donor Ligands journal August 1998
Cationic alkyl aluminium ethylene polymerization catalysts based on monoanionic N,N,N-pyridyliminoamide ligands journal January 1998

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