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Superconducting Tl-Ca-Ba-Cu-O thin films by reactive magnetron sputtering

Conference · · AIP Conference Proceedings (American Institute of Physics); (USA)
OSTI ID:7123054
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  1. Brookhaven National Laboratory, Upton, NY 11973 (USA)

Superconducting Tl-Ca-Ba-Cu-O thin films with T{sub c} onsets of 115 K and T{sub c} (R=0) of 95 K have been prepared by reactive magnetron sputtering using Tl, Cu and Ca/Ba metal targets. It was found that proper thallium content a is crucial for obtaining a high transition temperature. Wet oxygen and sealed gold tube with additional thallium compounds were used to reduce the loss of thallium during annealing. X-ray diffraction spectra show that films with the sharpest transition at 95 K are predominantly c-axis oriented. XANES also shows a preferred c-axis orientation for the superconducting films while for a nonsuperconducting film the near edge structure suggests greater disorder. X-ray microprobe fluorescence measurements indicate that these films are close to the 2122 stoichiometry. Scanning electron microscopy on these films is also presented.

DOE Contract Number:
AC02-76CH00016
OSTI ID:
7123054
Report Number(s):
CONF-881035--
Journal Information:
AIP Conference Proceedings (American Institute of Physics); (USA), Journal Name: AIP Conference Proceedings (American Institute of Physics); (USA) Vol. 182:1; ISSN APCPC; ISSN 0094-243X
Country of Publication:
United States
Language:
English