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(Li(Me sub 2 NCH sub 2 CH sub 2 NMe sub 2 ) sub 2 )(Li sub 2 (Me sub 2 CH sub 2 NMe sub 2 ) sub 2 -(. eta. -. nu. sup 5 ,. nu. sup 5 -MeC sub 5 H sub 4 ))((. eta. sup 5 -MeC sub 5 H sub 4 ) sub 6 U sub 2 (. mu. -Me)) sub 2 : A compound with symmetrically bridging MeC sub 5 H sub 4 and Me groups

Journal Article · · Journal of the American Chemical Society; (USA)
DOI:https://doi.org/10.1021/ja00194a060· OSTI ID:7073218
Organometallic compounds of the alkali metals which contain symmetrical bridging cyclopentadienyl groups, i.e., those in which two metal centers are located at equal distance on either side of and on the pseudo C{sub 5}-axis of the cyclopentadienyl group, are rare; the only example is the linear zigzag polymeric structure of (Na(Me{sub 2}NCH{sub 2}CH{sub 2}NMe{sub 2})Cp). The authors describe the synthesis and x-ray crystal structure of (Li-(Me{sub 2}NCH{sub 2}CH{sub 2}NMe{sub 2}){sub 2}){center dot}(Li(Me{sub 2}NCH{sub 2}CH{sub 2}NMe{sub 2})){sub 2}({mu}-MeC{sub 5}H{sub 4}){center dot}((MeC{sub 5}H{sub 4}){sub 3}U){sub 2}({mu}-Me), a compound that contains a MeC{sub 5}H{sub 4} group sandwiched between two Li(Me{sub 2}NCH{sub 2}CH{sub 2}NMe{sub 2}) fragments and a methyl group that is symmetrically bridging between two (MeC{sub 5}H{sub 4}){sub 3}U groups.
DOE Contract Number:
AC03-76SF00098
OSTI ID:
7073218
Journal Information:
Journal of the American Chemical Society; (USA), Journal Name: Journal of the American Chemical Society; (USA) Vol. 111:12; ISSN 0002-7863; ISSN JACSA
Country of Publication:
United States
Language:
English