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Cw laser ionization of C[sub 60] and C[sub 70]

Journal Article · · Physical Review Letters; (United States)
; ; ; ;  [1]
  1. Oak Ridge National Laboratory, P.O. Box 2008, Oak Ridge, Tennessee 37831-6125 (United States)
Delayed'' photoionization of the all-carbon cage fullerene molecules C[sub 60] and C[sub 70] is observed using a weakly focused cw argon ion laser (flux [ital I][lt]10[sup 5] W/cm[sup 2]). At these fluxes photoexcitation occurs incoherently and so slowly that intersystem crossing must be occurring simultaneously. A thermionic emission'' model adequately describes the delayed ionization.
DOE Contract Number:
AC05-84OR21400
OSTI ID:
6952795
Journal Information:
Physical Review Letters; (United States), Journal Name: Physical Review Letters; (United States) Vol. 73:8; ISSN 0031-9007; ISSN PRLTAO
Country of Publication:
United States
Language:
English