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Antiferromagnetic form factor of Sr sub 2 CuO sub 2 Cl sub 2

Journal Article · · Journal of Applied Physics; (USA)
DOI:https://doi.org/10.1063/1.344857· OSTI ID:6948123
; ; ; ; ;  [1]; ;  [2]
  1. Ames Laboratory, Ames, IA (USA) Physics Department, Iowa State University Ames, Iowa 50011 (USA)
  2. Argonne National Laboratory, Argonne, Illinois 60439 (USA)

Neutron diffraction techniques have been used to study the antiferromagnetic form factor of Sr{sub 2}CuO{sub 2}Cl{sub 2}, which has the body-centered-tetragonal ({ital I}4/{ital mmm}) K{sub 2}NiF{sub 4}-type structure (the same as that of tetragonal La{sub 2}CuO{sub 4} but with the out-of-plane oxygens replaced by Cl and the La by Sr). The antiferromagnetic form factor was obtained at 15 K by measuring the integrated intensities of the ( (1)/(2) (1)/(2) 0), ( (1)/(2) (1)/(2) 2), ( (1)/(2) (1)/(2) 3), ( (3)/(2) (3)/(2) 0), ( (3)/(2) (3)/(2) 6), ( (3)/(2) (5)/(2) 1), ( (3)/(2) (3)/(2) 8), and ( (5)/(2) (5)/(2) 0) magnetic reflections of a single crystal of Sr{sub 2}CuO{sub 2}Cl{sub 2}. The experimentally determined magnetic form factor is similar to that of La{sub 2}CuO{sub 4}. The experimental data were compared with the Cu{sup 2+} magnetic form factor and with the results of band theoretical calculations. We find that the fit to the experimental data is improved if one assumes a dipolar spin polarization on the in-plane oxygen ions.

OSTI ID:
6948123
Journal Information:
Journal of Applied Physics; (USA), Journal Name: Journal of Applied Physics; (USA) Vol. 67:9; ISSN 0021-8979; ISSN JAPIA
Country of Publication:
United States
Language:
English