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Neutron-diffraction study of the antiferromagnetic form factor of La sub 2 NiO sub 4

Journal Article · · Physical Review, B: Condensed Matter; (United States)
; ; ; ; ;  [1];  [2]; ;  [3];  [4]
  1. Ames Laboratory and Department of Physics, Iowa State University, Ames, Iowa 50011 (United States)
  2. Commission of European Communities, Joint Research Center, Postfach 2340, D-7500 Karlsruhe (Germany)
  3. Argonne National Laboratory, Argonne, Illinois 60439 (United States)
  4. Department of Chemistry, Purdue University, West Lafayette, Indiana 47907 (United States)

Neutron-diffraction techniques have been used to study the antiferromagnetic form factor of a La{sub 2}NiO{sub 4} single crystal at 15 K. The antiferromagnetic form factor was obtained by measuring the integrated intensities of 16 magnetic reflections. A plateau is clearly seen at low {ital Q} (up to 3 A{sup {minus}1}) in the experimentally determined form factor, similar to those observed for La{sub 2}CuO{sub 4} and Sr{sub 2}CuO{sub 2}Cl{sub 2}. The magnetization density deduced from the experimental data exhibits strong ansiotropy in the Ni-O plane. The experimental data are compared with covalency models and a recent spin-polarized band calculation.

DOE Contract Number:
W-7405-ENG-82; W-31109-ENG-38; FG02-90ER45427
OSTI ID:
5001559
Journal Information:
Physical Review, B: Condensed Matter; (United States), Journal Name: Physical Review, B: Condensed Matter; (United States) Vol. 45:10; ISSN 0163-1829; ISSN PRBMD
Country of Publication:
United States
Language:
English