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Theory of screening and electron mobility: Application to [ital n]-type silicon

Journal Article · · Physical Review, B: Condensed Matter; (United States)
;  [1];  [2]
  1. Department of Physics, State University of New York at Stony Brook, Stony Brook, New York 11794-3800 (United States)
  2. Department of Physics and Astronomy, The University of Tennessee, Knoxville, Tennessee 37996-1200 (United States) Solid State Division, Oak Ridge National Laboratory, P.O. Box 2008, Oak Ridge, Tennessee 37831-6030 (United States)

The dielectric function for semidegenerate [ital n]-type silicon is calculated in both the random-phase approximation (RPA) and the Singwi-Tosi-Land-Sjoelander (STLS) approximation in a study of linear screening theory and electron mobility. Using a spherical effective-mass model for the six conduction-band valleys, the Boltzmann equation is solved exactly for phonon plus impurity scattering and the resulting mobility is compared with experiment. Significant differences are found in doped silicon at nonzero temperatures between Boltzmann equation solutions in the RPA Born approximation and the less accurate force-force correlation function formula for the electrical resistivity due to electron-impurity scattering. Phonon scattering has only secondary importance and is treated by standard deformation-potential models. The problem of scattering by linearly screened ionized impurities is treated with exact phase-shift scattering theory. RPA phase-shift calculated electron mobilities in [ital n]-type silicon at 300 and 77 K agree more closely with experiment than the Born approximation or Thomas-Fermi calculations. The local field correction to RPA screening of impurity potentials is not significant in scattering cross sections when the electron-electron vertex function is included. However, assuming full ionization, the STLS dielectric function yields negative electronic compressibilities at 77 K in a concentration region centered approximately where the metal-insulator transition takes place at [ital T]=0, and coinciding with strong violations of the Friedel sum rule by linearly screened potentials. Strong Coulomb interactions are indicated and imply an inadequacy of linear screening theory, the Born approximation, and the Boltzmann equation for electron-impurity scattering applied to the electron-gas model for doped silicon at low temperature, despite apparently good agreement with experiment.

DOE Contract Number:
AC05-84OR21400
OSTI ID:
6906003
Journal Information:
Physical Review, B: Condensed Matter; (United States), Journal Name: Physical Review, B: Condensed Matter; (United States) Vol. 46:23; ISSN 0163-1829; ISSN PRBMDO
Country of Publication:
United States
Language:
English