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235U(n,f), 238U(n,$$\gamma$$), 238U(n,f), and 238Pu(n,f) Reaction Rate Measurement Calibrations at ZPPR

Technical Report ·
DOI:https://doi.org/10.2172/6819232· OSTI ID:6819232

New reference deposits for 235U, 239Pu and 238U have been established with mass uncertainties of <0.2%. These new deposits replace the older reference deposits which were used during the last 17 years and improve the uncertainty of reaction rate measurements due to reference mass uncertainties by about a factor of 6. Measurements of the fission fragment absorption in 2π geometry have been made for these deposits using a new technique of comparing 2π and low-geometry count rates. Two measurements of the 238U capture rate in depleted uranium samples based upon the thermal cross sections of 238U(n,$$\gamma$$), 235U(n,f) and 239Pu(n,f) and based upon the 243Am calibration technique confirm the ZPPR measurement technique within the quoted uncertainty of ±0.5%.

Research Organization:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA), Nuclear Criticality Safety Program (NCSP)
DOE Contract Number:
W-31109-ENG-38
OSTI ID:
6819232
Report Number(s):
ANL-87-5; ON: DE87005942
Country of Publication:
United States
Language:
English