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Appearance potentials of positive ions produced by electron-impact dissociative ionization of SF{sub 6}, SF{sub 5}Cl, S{sub 2}F{sub 10}, and SOF{sub 2}

Journal Article · · Bulletin of the American Physical Society
OSTI ID:67897

Appearance potentials (APs) of positive ions produced in the ion source of a quadrupole mass spectrometer by electron collision with the molecules SF{sub 6}, SF{sub 5}Cl, S{sub 2}F{sub 10}, and SOF{sub 2} are measured. The electron-energy scale is calibrated by comparing the ion onset energies with the observed onset of Ar{sup +} from argon mixed with the sample gases. The APs of the fragment ions from SF{sub 6} are in agreement with previous results. In the case of S{sub 2}F{sub 10}, which has a mass spectrum at 70 eV nearly identical to that of SF{sub 6}, the APs of the predominant fragment ions are found to be significantly lower than the corresponding ions from SF{sub 6}, e.g., SF{sub 5}{sup +} and SF{sub 3}{sup +} appear respectively at 13.2 and 13.3 eV from S{sub 2}F{sub 10} and at 15.7 and 19.7 eV from SF{sub 6}. The relevance of these results to the use of mass spectrometry for detection of discharge by-products in SF{sub 6} is discussed.

OSTI ID:
67897
Report Number(s):
CONF-9310400--
Journal Information:
Bulletin of the American Physical Society, Journal Name: Bulletin of the American Physical Society Journal Issue: 13 Vol. 38; ISSN BAPSA6; ISSN 0003-0503
Country of Publication:
United States
Language:
English

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