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Generation of alkylarsines from soil

Journal Article · · Weed Sci.; (United States)
OSTI ID:6484034

Products volatilized from arsenical-treated soil were identified and their rates of formation measured to determined if generation of alkylarsines by soils is part of a natural arsenic cycle. As-sodium arsenate, /sup 14/C-MSMA (monosodium methanearsonate), or /sup 14/C-cacodylic acid (hydroxydimethylarsine oxide), were added at 13.3 ..mu..Moles (10 ppmw As) to individual flasks containing 100 g of Mattapeake silt loam. Volatile arsine gases were produced under all conditions. The organo-arsenicals formed volatile compounds most quickly under aerobic conditions. The volatile gases were identified as dimethyl- and trimethylarsine (DMA and TMA) by ion exchange and gas chromatography, and mass spectroscopy. Most of the extractable arsenic remaining in the soil was present as a trimethyl arsenical compound regardless of the treatment. Since arsenic was transferred to air regardless of arsenical treatment, the transfer of arsenic from soil to air is part of the natural arsenic cycle in soils.

Research Organization:
Dept. of Agriculture, Beltsville, MD
OSTI ID:
6484034
Journal Information:
Weed Sci.; (United States), Journal Name: Weed Sci.; (United States) Vol. 25:5; ISSN WEESA
Country of Publication:
United States
Language:
English

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