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X-ray spectroscopic investigation of metamictization and annealing in crystalline phosphates, silicates and complex Ti-Nb-Ta oxides. Final report

Technical Report ·
OSTI ID:6442467
Metamict minerals have been damaged by the radioactive decay of their U and Th components and have been exposed to geologic processes over periods of many hundreds of millions of years. These metamict minerals can be considered to be the products of a natural long-term radiation damage experiment, hence there will be increased interest in the long term stability of these minerals because of their crystal-chemical similarities with phases in proposed waste-forms. A study was initiated of the effects of metamictization and annealing on crystalline phosphates, silicates and complex A/sub x/B/sub y/O/sub z/-type Ti-Nb-Ta oxides. This study included a detailed examination of the near neighbor site geometries of metal atoms in metamict minerals (e.g., A (Ca) and B (Ti) site cations) as determined by extended x-ray absorption fine structure (EXAFS) and x-ray absorption near edge structure (XANES) spectroscopy.
Research Organization:
Boeing Aerospace Co., Seattle, WA (USA)
DOE Contract Number:
AC06-83ER45010
OSTI ID:
6442467
Report Number(s):
DOE/ER/45010-T1; ON: DE85000428
Country of Publication:
United States
Language:
English