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Thermal behavior of shell molybdena-alumina catalysts

Journal Article · · AIChE Symp. Ser.; (United States)
Heat treatment of ''shell'' molybdena-alumina catalyst pellets results in macroscopic redistribution of the molybdena. Redistribution is minimal at 625/sup 0/C but extensive at 750/sup 0/C. After 6 hours at 750/sup 0/, a sharp maximum is observed in the radial distribution. This is a result of opposing factors: radial diffusion inward from the initial shell, and preferential sintering of the alumina support in the shell region. Loss of molybdena by vaporization is not appreciable at 750/sup 0/C but is serious at 875/sup 0/C. A computer program has been developed to convert SEM-EDAX (scanning electron microscopy energy-dispersive analysis of x-ray) data for unpolished pellet sections to a quantitative, smooth profile of Mo concentration as a function of reduced radial position.
Research Organization:
Department of Chemical Engineering, State University of New York at Buffalo, Buffalo, NY
OSTI ID:
6264817
Journal Information:
AIChE Symp. Ser.; (United States), Journal Name: AIChE Symp. Ser.; (United States) Vol. 31:3; ISSN ACSSC
Country of Publication:
United States
Language:
English