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Generation of binuclear (d/sup 8/. d/sup 8/)psigma platinum and rhodium complexes by pulse radiolysis

Journal Article · · J. Am. Chem. Soc.; (United States)
DOI:https://doi.org/10.1021/ja00330a018· OSTI ID:6199691

Two (d/sup 8/.d/sup 8/)psigma binuclear complexes, Pt/sub 2/(pop)/sub 4//sup 5 -/ (pop = P/sub 2/O/sub 5/H/sub 2//sup 2 -/) and Rh/sub 2/(TMB)/sub 4//sup +/ (TMB = 2,5-dimethyl-2,5-diisocyanohexane), have been generated by pulse radiolysis of aqueous and acetonitrile solutions, respectively, of the corresponding d/sup 8/.d/sup 8/ species. An intense absorption system attributable to the allowed dsigma* ..-->.. psigma transition is observed in the spectrum of each of the transients (420 nm, Pt/sub 2/(pop)/sub 4//sup 5 -/; 570 nm, Rh/sub 2/(TMB)/sub 4//sup +/).

Research Organization:
California Inst. of Tech., Pasadena
OSTI ID:
6199691
Journal Information:
J. Am. Chem. Soc.; (United States), Journal Name: J. Am. Chem. Soc.; (United States) Vol. 106:18; ISSN JACSA
Country of Publication:
United States
Language:
English