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Systematic determination of extended atomic orbital basis sets and application to molecular SCF and MCSCF calculations

Technical Report ·
DOI:https://doi.org/10.2172/6161362· OSTI ID:6161362
The behavior of the two exponential parameters in an even-tempered gaussian basis set is investigated as the set optimally approaches an integral transform representation of the radial portion of atomic and molecular orbitals. This approach permits a highly accurate assessment of the Hartree-Fock limit for atoms and molecules.
Research Organization:
Ames Lab., IA (USA)
DOE Contract Number:
W-7405-ENG-82
OSTI ID:
6161362
Report Number(s):
IS-T-852
Country of Publication:
United States
Language:
English

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