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Oxidative addition of H/sub 2/ to the A-frame complex (Tr/sub 2/(CO)/sub 2/(. mu. -S)(Ph/sub 2/PCH/sub 2/PPh/sub 2/)/sub 2/): a reinvestigation

Journal Article · · Inorg. Chem.; (United States)
DOI:https://doi.org/10.1021/ic00293a048· OSTI ID:6084796
A reinvestigation of the reaction of the A-frame complex (Ir/sub 2/(CO)/sub 2/(..mu..-S)(DPPM)/sub 2/) (DPPM = Ph/sub 2/PCH/sub 2/PPh/sub 2/) with H/sub 2/ using improved spectroscopic techniques is reported herein. It is proposed that the reaction is an oxidative addition of H/sub 2/ at one metal center followed by transfer of one hydride ligand to the other metal and concomitant Ir-Ir bond formation. 23 references, 1 figure, 1 table.
Research Organization:
Univ. of Alberta, Edmonton (Canada)
OSTI ID:
6084796
Journal Information:
Inorg. Chem.; (United States), Journal Name: Inorg. Chem.; (United States) Vol. 27:20; ISSN INOCA
Country of Publication:
United States
Language:
English