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Synthesis, rapid resolution, and determination of absolute configuration of racemic 2,2'-binaphthyldiyl crown ethers and analogues via. beta. -cyclodextrin complexation

Journal Article · · J. Org. Chem.; (United States)
DOI:https://doi.org/10.1021/jo00350a025· OSTI ID:6036624

Twenty racemic and four diastereomeric 2,2'-binaphthyldiyl crown ethers and analogues were synthesized. Chiral interactions between these compounds and immobilized ..beta..-cyclodextrin were examined. Thirteen of the enantiometic pairs and two of the diastereomers were successfully resolved. It was found that relatively small changes in the structure of these compounds could have large effects on chiral recognition. In general, the (-)-S enantiomers formed stronger inclusion complexes with ..beta..-cyclodextrin than did the (+)-R enantiomers. 40 references, 2 figures, 2 tables.

Research Organization:
Texas Tech Univ., Lubbock
DOE Contract Number:
AS05-84ER13159
OSTI ID:
6036624
Journal Information:
J. Org. Chem.; (United States), Journal Name: J. Org. Chem.; (United States) Vol. 50:26; ISSN JOCEA
Country of Publication:
United States
Language:
English