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Photoelectron diffraction k-space volumes of the c(2x2) Mn/Ni(100) structure

Technical Report ·
DOI:https://doi.org/10.2172/603530· OSTI ID:603530
; ;  [1]
  1. Univ. of Wisconsin, Milwaukee, WI (United States); and others

Traditionally, x-ray photoelectron diffraction (XPD) studies have either been done by scanning the diffraction angle for fixed kinetic energy (ADPD), or scanning the kinetic energy at fixed exit angle (EDPD). Both of these methods collect subsets of the full diffraction pattern, or volume, which is the intensity of photoemission as a function of momentum direction and magnitude. With the high density available at the Spectromicroscopy Facility (BL 7.0) {open_quotes}ultraESCA{close_quotes} station, the authors are able to completely characterize the photoelectron diffraction patterns of surface structures, up to several hundred electron volts kinetic energy. This large diffraction `volume` can then be analyzed in many ways. The k-space volume contains as a subset the energy dependent photoelectron diffraction spectra along all emission angles. It also contains individual, hemispherical, diffraction patterns at specific kinetic energies. Other `cuts` through the data set are also possible, revealing new ways of viewing photoelectron diffraction data, and potentially new information about the surface structure being studied. In this article the authors report a brief summary of a structural study being done on the c(2x2) Mn/Ni(100) surface alloy. This system is interesting for both structural and magnetic reasons. Magnetically, the Mn/Ni(100) surface alloy exhibits parallel coupling of the Mn and Ni moments, which is opposite to the reported coupling for the bulk, disordered, alloy. Structurally, the Mn atoms are believed to lie well above the surface plane.

Research Organization:
Lawrence Berkeley Lab., CA (United States)
DOE Contract Number:
FG02-92ER45468
OSTI ID:
603530
Report Number(s):
LBNL--39981; ON: DE97007345; CNN: Grant DMR-9413475
Country of Publication:
United States
Language:
English