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Cosmogenic neutron-capture-produced nuclides in stony meteorites

Journal Article · · J. Geophys. Res.; (United States)

The distribution of neutrons with energies below 15 MeV in spherical stony meteoroids is calculated using the ANISN neutron-transport code. The source distributions and intensities of neutrons are calculated using cross sections for the production of tritium. The meteoroid's radius and chemical composition strongly influence the total neutron flux and the neutron energy spectrum, whereas the location within a meteoroid only affects the relative neutron intensities. Meteoroids must have radii of more than 50 g/cm/sup 2/ before they have appreciable fluxes of neutrons near thermal energies. Meteoroids with high hydrogen or low iron contents can thermalize neutrons better than chondrites can. Rates for the production of /sup 60/Co, /sup 59/Ni, and /sup 36/Cl are calculated with these neutron fluxes and evaluated neutron-capture cross sections and are reported for carbonaceous chondrites with high hydrogen contents, L-chondrites, and aubrites. For most meteoroids with radii <300 g/cm/sup 2/, the production rates of these neutron-capture nuclides increase monotonically with depth. The highest calculated /sup 60/Co production rate in an ordinary chondrite is 375 atoms/min/g-Co at the center of a meteoroid with a 250 g/cm/sup 2/ radius. The production rates calculated for spallogenic /sup 60/Co and /sup 59/Ni are greater than the neutron-capture rates for radii less than approx.50-75 g/cm/sup 2/. Only for very large meteoroids and chlorine-rich samples is the neutron-capture production of /sup 36/Cl important. The results of these calculations are compared with those of previous calculations and with measured activities in many meteorites.

Research Organization:
Department of Natural Science, York College of C.U.N.Y.
OSTI ID:
5939468
Journal Information:
J. Geophys. Res.; (United States), Journal Name: J. Geophys. Res.; (United States) Vol. 91:B4; ISSN JGREA
Country of Publication:
United States
Language:
English