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Reactive and inelastic energy transfer in H+D/sub 2/ collisions studied by single-collision CARS spectroscopy

Conference ·
OSTI ID:5880776
;
Highly time-resolved (approx. =5ns) coherent anti-Stokes Raman scattering (CARS) spectroscopy obtains product Raman spectra after single collisions with D/sub 2/ of laser-photolytically-generated hydrogen atoms. Varying photolysis wavelength changes H-atom energies. HD and D/sub 2/ Raman spectra yield product quantum-state distributions, elucidating dynamics of reactive and inelastic energy transfer.
OSTI ID:
5880776
Report Number(s):
CONF-841121-
Country of Publication:
United States
Language:
English

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Related Subjects

640304* -- Atomic
Molecular & Chemical Physics-- Collision Phenomena
74 ATOMIC AND MOLECULAR PHYSICS
ATOM COLLISIONS
ATOM-ATOM COLLISIONS
CHEMICAL REACTIONS
COLLISIONS
DECOMPOSITION
DEUTERIDES
DEUTERIUM
DEUTERIUM COMPOUNDS
DYNAMICS
ELEMENTS
ENERGY TRANSFER
HYDROGEN
HYDROGEN COMPOUNDS
HYDROGEN ISOTOPES
ISOTOPES
LASER SPECTROSCOPY
LASERS
LIGHT NUCLEI
MECHANICS
NONMETALS
NUCLEI
ODD-ODD NUCLEI
PHOTOCHEMICAL REACTIONS
PHOTOLYSIS
RAMAN SPECTROSCOPY
SPECTROSCOPY
STABLE ISOTOPES
WAVELENGTHS