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Structural and magnetic properties of UCo sub 2 Ge sub 2

Journal Article · · Journal of Applied Physics; (USA)
DOI:https://doi.org/10.1063/1.348240· OSTI ID:5694959
; ; ;  [1]
  1. Kamerlingh Onnes Laboratorium der Rijksuniversiteit Leiden, P.O. Box 9506, 2300 RA Leiden, The Netherlands (NL)
We have studied the effect of annealing on the structural and magnetic properties of UCo{sub 2}Ge{sub 2} and thereby find the existence of two different crystallographic structures. The as-cast, high-temperature (HT) phase adopts a crystal structure with symmetry lower than {ital I}4/{ital mmm}; after annealing at 750 {degree}C for 5 days the ThCr{sub 2}Si{sub 2} ({ital I}4/{ital mmm}) structure is formed. Additionally, the length of the {ital c} axis in these tetragonal structures changes dramatically: whereas the HT phase has a {ital c} parameter of {approx}9.3 A, the low-temperature (LT), annealed phase has a much larger {ital c} axis of {approx}9.9 A. This expansion of the unit cell greatly influences the magnetic properties of the material: while the LT sample orders antiferromagnetically at 174 K, the HT one does not order magnetically down to 350 mK. The antiferromagnetic transition is clearly indicated by our magnetization, resistivity and specific heat measurements.
OSTI ID:
5694959
Journal Information:
Journal of Applied Physics; (USA), Journal Name: Journal of Applied Physics; (USA) Vol. 69:8; ISSN 0021-8979; ISSN JAPIA
Country of Publication:
United States
Language:
English