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U.S. Department of Energy
Office of Scientific and Technical Information

Implications of a gradient in acid and ion deposition across the northern Great Lakes states

Technical Report ·
OSTI ID:5594447
Average precipitation pH, 1979-1982, declines from west to east from 5.3 to 4.3 along a cross section of sites in Minnesota, Wisconsin, and Michigan. This answers questions about the seasonal and geographic pattern of anthropogenic acid precursor emissions and reaction products (SO/sub 4//sup -2/, NO/sub 3//sup -/, H/sup +/, NH/sub 4//sup +/) that increase from west to east. Except for higher concentrations of Ca/sup 2 +/ and Mg/sup 2 +/ observed at one site in the cultivated area of southwestern Minnesota, the contribution of soil-related metal cations to the total ions in solution is small (17%) and relatively uniform across the region. Significant seasonal and geographic patterns in precipitation chemistry and deposition values are observed. Close correspondence of the sums of strong acid anions with the sums of hydrogen and ammonium ions in precipitation is observed, indicating anthropogenic sources of sulfur and nitrogen oxides.
Research Organization:
Environmental Protection Agency, Duluth, MN (USA). Environmental Research Lab.
OSTI ID:
5594447
Report Number(s):
PB-86-176062/XAB; EPA/600/J-86/002
Country of Publication:
United States
Language:
English