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U.S. Department of Energy
Office of Scientific and Technical Information

Atmospheric trace gases over China

Journal Article · · Environ. Sci. Technol.; (United States)
DOI:https://doi.org/10.1021/es00096a014· OSTI ID:5581565

Flask sampling, EC/GC, and FID/GC techniques were used to measure the concentrations of CO, CH/sub 4/, CH/sub 3/,Cl, N/sub 2/O, CCl/sub 4/, CH/sub 3/CCl/sub 3/, CCl/sub 3/F, CCl/sub 2/F, and CHClF/sub 2/ in the air over four urban and three rural areas in the People's Republic of China. The results were compared with the concentrations of these trace gases found over urban and rural areas of Oregon, U.S.A. More CCl/sub 4/ and CH were found over Chinese cities than over Oregon cities or over rural China. CO, CH/sub 3/Cl, N/sub 2/O and CH/sub 4/ were all significantly more abundant over rural China than over the clean background site in Oregon. In China rural sources of CO and CH/sub 3/Cl include smoldering combustion in homes, whereas rice paddies and biogas conversion may be sources of CH/sub 4/. Our results show that China may have significant anthropogenic sources of CH/sub 4/, N/sub 2/O, and CCl/sub 4/, all of which are increasing in the atmosphere and may alter the earth's climate if their increases continue for a long time.

OSTI ID:
5581565
Journal Information:
Environ. Sci. Technol.; (United States), Journal Name: Environ. Sci. Technol.; (United States) Vol. 16:2; ISSN ESTHA
Country of Publication:
United States
Language:
English