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Peculiar low-temperature properties of metallic Nd{sub 2{minus}x}Ce{sub x}CuO{sub 4} caused by interactions between Nd moments and conduction electrons

Journal Article · · Physical Review, B: Condensed Matter
; ; ; ; ;  [1]; ;  [2]
  1. Forschungszentrum Karlsruhe, Institut fuer Nukleare Festkoerperphysik, P.O. Box 3640, D-76021 Karlsruhe (Germany)
  2. Center for Superconductivity Research, Department of Physics, University of Maryland, College Park, Maryland 20742-4111 (United States)

Low-energy magnetic excitations in Nd{sub 2{minus}x}Ce{sub x}CuO{sub 4} with 0{le}x{le}0.2 have been investigated by measurements of the specific heat. For all Ce-doped samples (x{ge}0.05), a linear term {gamma}T was found at very low temperatures (T{approx_lt}0.5K), with 0.3J/K{sup 2}{approx_lt}{gamma}{approx_lt}0.6J/K{sup 2} per mole Nd for 0.05{le}x{lt}0.14, and 3J/K{sup 2}{approx_lt}{gamma}{approx_lt}4J/K{sup 2} per mole Nd for higher Ce concentrations. In overdoped Nd{sub 1.8}Ce{sub 0.2}CuO{sub 4}, {gamma} is rapidly suppressed in magnetic fields exceeding 1.5 T. The temperature dependence of the electrical resistance parallel to the CuO{sub 2} planes corresponds to that of two-dimensional metals. The magnetoresistance of Nd{sub 1.8}Ce{sub 0.2}CuO{sub 4} single crystals and c-axis-oriented thin films in magnetic fields parallel to the CuO{sub 2} planes is monotonously negative at temperatures above 1 K. Below about 500 mK, the magnetoresistance is positive in small fields, it goes through a maximum near 2 T, and it is negative for B{gt}2T. These features are similar to those observed in heavy-fermion systems. In contrast, in Pr{sub 1.8}Ce{sub 0.2}CuO{sub 4}, with nonmagnetic Pr, the magnetoresistance is negative at all temperatures of our measurements down to 20 mK. This proves unambiguously that interactions between conduction electrons and Nd moments give rise to the low-temperature maximum of the magnetoresistance. Furthermore, a comparison of the magnetoresistance with the modification of the specific heat by magnetic fields supports the interpretation of the large linear term as resulting from the interaction between Nd moments and conduction electrons. {copyright} {ital 1997} {ital The American Physical Society}

OSTI ID:
553099
Journal Information:
Physical Review, B: Condensed Matter, Journal Name: Physical Review, B: Condensed Matter Journal Issue: 20 Vol. 56; ISSN 0163-1829; ISSN PRBMDO
Country of Publication:
United States
Language:
English

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