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U.S. Department of Energy
Office of Scientific and Technical Information

Investigation of vaporization and devolatilization of coal/water mixtures. Sixth quarterly report, August 1-October 31, 1983

Technical Report ·
OSTI ID:5433397

The objective of this program is to develop the capabilities to predict the vaporization and devolatilization behavior of coal/water mixtures under conditions appropriate for spray combustion. The program is currently collecting data in an entrained flow coal reactor which has a fixed position, coal/water slurry spray injector and a movable product extractor. This reactor is being used to study the vaporization and pyrolysis of coal/water slurries. FT-IR is used for the analysis of the product gases, tars and chars to determine species evolution kinetics and kinetics of secondary reactions such as steam-char reactions, cracking, soot formation, char gasification, censophere formation and particle swelling, and char reactivity. Pyrolysis calculations have been performed to compare with the data for the Pittsburgh Seam coal/water slurry collected in the reactor system at furnace temperatures of 1100/sup 0/C and 1300/sup 0/C. The general behavior of the various species indicates more conversion of aliphatics to CO and CO/sub 2/, compared to dry coal pyrolysis. Chars from slurry pyrolyses at 1100/sup 0/C and 1300/sup 0/C show substantial agglomeration.

Research Organization:
Advanced Fuel Research, Inc., East Hartford, CT (USA)
DOE Contract Number:
AC22-82PC50254
OSTI ID:
5433397
Report Number(s):
DOE/PC/50254-T6; ON: DE84005260
Country of Publication:
United States
Language:
English