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Atmospheric reactive nitrogen: A model study of natural and anthropogenic sources and the role of microbial soil emissions

Conference ·
OSTI ID:5387719
Nitrogen oxides (NO{sub x} = NO + NO{sub 2}) are primary pollutants which react in the atmosphere to form nitric acid (HNO{sub 3}). Nitric acid is a major contributor to acid wet and dry deposition and can also affect the reactive nitrogen nutrients in soil and ocean ecosystems. In addition, NO{sub x} takes part in the photochemical cycle of ozone (O{sub 3}). Tropospheric O{sub 3} is important from both an atmospheric and a biological perspective. It acts as a greenhouse gas warming the earth's surface and as a chemical oxidant which can cause injury to humans, plants, and animals. Anthropogenic sources including 22 Tg N from fossil fuel burning and 5-13 Tg N from biomass burning constitute the largest contribution (Tg=10{sup 12}g). Less is understood abut the natural sources of NO{sub x} and in particular the emissions from microbial activity in soils. Here we present a model calculated, seasonally and spatially resolved (1 {times} 1 degree), inventory of the annual soil emissions of NO{sub x} from microbial activity from natural vegetation ecosystems. The soil emissions model addresses the emissions of soils from the natural vegetation types. Emissions from soil microbial activity have been shown to be temperature and moisture dependent.
Research Organization:
Lawrence Livermore National Lab., CA (United States)
Sponsoring Organization:
DOE; USDOE, Washington, DC (United States)
DOE Contract Number:
W-7405-ENG-48
OSTI ID:
5387719
Report Number(s):
UCRL-JC-107393; CONF-911212--1; ON: DE92010717
Country of Publication:
United States
Language:
English