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Development of CNDO/2 for calculation of the structure of compounds of third period elements

Journal Article · · Dokl. Phys. Chem. (Engl. Transl.); (United States)
OSTI ID:5377351

The authors developed a version of CNDO/2 for the calculation of the electronic structure, the geometry, and other parameters of compounds of third period elements, which is to a considerable degree free from the shortcomings of the other methods. In this version the 3d AOs are included in the basis set and the dependence of the exponent on the electronic structure of the atom is taken into account by optimizing the Slater exponents of the 3d AOs of the third period atoms using the minimum total energy criteria. They used Gordon's exponents for the 3s and 3p AOs. This version was tested on a large series of inorganic and organic phosphorus compounds.

Research Organization:
Lomonosov Moscow State Univ. (USSR)
OSTI ID:
5377351
Journal Information:
Dokl. Phys. Chem. (Engl. Transl.); (United States), Journal Name: Dokl. Phys. Chem. (Engl. Transl.); (United States) Vol. 292:1/3; ISSN DKPCA
Country of Publication:
United States
Language:
English