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Title: Neutron capture studies: 1, Multiple capture reactions and implications for calculated beta-delayed fission rates: 2, The nuclear level structure of 238Np

Conference ·
OSTI ID:5291231

Astrophysical r-process calculations of transbismuth elements are of interest because certain actinide pairs can be treated as chronometers in determining the duration of nucleosynthesis. For one such calculation where a particularly long galactic age was derived, 21 + 2 - 4 Gyr, we present evidence that the effect of beta-delayed fission appears to be seriously overestimated in uranium decay chains with A = 252 to 257. With this conclusion, it follows that this estimate of the galactic age must be considered more uncertain than if the calculated rates of beta-delayed fission were found to be acceptable. The nuclear level structure of 238Np has been investigated using the 237Np(n,..gamma..)238Np reaction and the alpha decay of 242mAm as experimental probes. Having established a level scheme for 238Np that includes 47 excited levels and 93 secondary transitions, we find a high degree of correspondence between the experimental band structure and that of a semi-empirical model developed to predict excitations in odd-odd deformed nuclei. 35 refs., 4 figs., 3 tabs.

Research Organization:
Lawrence Livermore National Lab., CA (USA)
DOE Contract Number:
W-7405-ENG-48
OSTI ID:
5291231
Report Number(s):
UCRL-97056; CONF-8708101-15; ON: DE88006577
Resource Relation:
Conference: 6. international symposium on capture gamma-ray spectroscopy, Leuven, Belgium, 31 Aug 1987; Other Information: Portions of this document are illegible in microfiche products
Country of Publication:
United States
Language:
English