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Beta-delayed fission and neutron emission calculations for the actinide cosmochronometers

Journal Article · · Phys. Rev. C; (United States)
The Gamow-Teller beta-strength distributions for 19 neutron-rich nuclei, including ten of interest for the production of the actinide cosmochronometers, are computed microscopically with a code that treats nuclear deformation explicitly. The strength distributions are then used to calculate the beta-delayed fission, neutron emission, and gamma deexcitation probabilities for these nuclei. Fission is treated both in the complete damping and WKB approximations for penetrabilities through the nuclear potential-energy surface. The resulting fission probabilities differ by factors of 2 to 3 or more from the results of previous calculations using microscopically computed beta-strength distributions around the region of greatest interest for production of the cosmochronometers. The indications are that a consistent treatment of nuclear deformation, fission barriers, and beta-strength functions is important in the calculation of delayed fission probabilities and the production of the actinide cosmochronometers. Since we show that the results are very sensitive to relatively small changes in model assumptions, large chronometric ages for the Galaxy based upon high beta-delayed fission probabilities derived from an inconsistent set of nuclear data calculations must be considered quite uncertain.
Research Organization:
Lawrence Livermore National Laboratory, Livermore, California 94550
DOE Contract Number:
W-7405-ENG-48
OSTI ID:
6068953
Journal Information:
Phys. Rev. C; (United States), Journal Name: Phys. Rev. C; (United States) Vol. 39:5; ISSN PRVCA
Country of Publication:
United States
Language:
English