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Observation of the new neutron-rich nuclide [sup 208]Hg

Journal Article · · Physical Review, C (Nuclear Physics); (United States)

The new neutron-rich isotope [sup 208]Hg was observed for the first time in the reaction products from a thick [sup nat]Pb target bombarded by a 30 MeV/nucleon [sup 12]C beam. A high efficiency release, separation, and collection of Hg products were of success with a good selectivity by using a special off-line gas-phase thermochromatographic process followed by a liquid-liquid procedure which was developed in the present work. The assignment of [sup 208]Hg was based on the identification of its [beta][sup [minus]] decay daughter [sup 208]Tl observed in the periodically extracted Tl element sample growing in the separated Hg element product solution. In the [gamma] spectra of the Tl samples a 2614.6-keV [gamma] activity with a half-life 191[sub [minus]50][sup +104] s was observed, which could only be assigned to the daughter [sup 208]Tl of [sup 208]Hg [beta][sup [minus]] decay. The measured [sup 208]Hg half-life was 42[sub [minus]12][sup +23] min and the average production cross section for the energy of the [sup 12]C beam ranging from 30 MeV/nucleon to 5 MeV/nucleon and the effective target thickness of 670 mg/cm[sup 2] was deduced to be 1.1[sub [minus]0.5][sup +1.0] [mu]b. Moreover, in the time-successive [gamma] spectra of the separated Hg sample, a 473.5-keV [gamma] activity corresponding to the [gamma] transition of 4[sup +] to ground state (5[sup +]) of [sup 208]Tl was observed and found to have the same half-life as the [sup 208]Hg [beta][sup [minus]] decay within the error range of the present work. A theoretical discussion for the obtained half-life of [sup 208]Hg is given.

OSTI ID:
5263653
Journal Information:
Physical Review, C (Nuclear Physics); (United States), Journal Name: Physical Review, C (Nuclear Physics); (United States) Vol. 49:2; ISSN 0556-2813; ISSN PRVCAN
Country of Publication:
United States
Language:
English