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Nonlinearity of the refractive index due to an excitonic molecule resonance state in CdS

Journal Article · · IEEE J. Quant. Electron.; (United States)
The authors report the observation of an intensity-dependent refractive-index nonlinearity in CdS due to a resonance state where an excitonic molecule is created by induced absorption of light. The refractive index n as a function of the incident laser photon energy E is measured directly by light refraction in thin crystal prisms. A renormalized dielectric function describes the measured n(E) spectra well. This strong refractive-index nonlinearity is well suited to produce an optical bistability and to further strengthen the evidence of CdS to be an important material for laser-induced dynamic gratings.
Research Organization:
Spectra Physics, Darmstadt
OSTI ID:
5243609
Journal Information:
IEEE J. Quant. Electron.; (United States), Journal Name: IEEE J. Quant. Electron.; (United States) Vol. QE-22:8; ISSN IEJQA
Country of Publication:
United States
Language:
English