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Third-harmonic generation and multiphoton ionizaton in rare gases

Journal Article · · Phys. Rev. A; (United States)

Resonantly enhanced multiphoton ionization (MPI) and third-harmonic generation (THG) have been concurrently studied in the rare gases, xenon, krypton, and argon. The disappearance with increasing pressure of the MPI signals resonant with the three-photon allowed 6s 5s, and 4s states, respectively, of the rare gases, is linked to the appearance of THG. Conversely, THG is shown to be partially quenched at certain wavelengths by one- and two-photon absorption leading to ionization.

Research Organization:
Chemical Physics Section, Health and Safety Research Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830
OSTI ID:
5233143
Journal Information:
Phys. Rev. A; (United States), Journal Name: Phys. Rev. A; (United States) Vol. 25:4; ISSN PLRAA
Country of Publication:
United States
Language:
English