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Independent yields from the photofission of sup 232 Th, and the Z sub p and statistical-dynamic models

Journal Article · · Physical Review, C (Nuclear Physics); (United States)
;  [1]
  1. Department of Chemistry, New Mexico State University, Las Cruces, New Mexico (USA)
Independent fission yields were measured for {sup 82}Br, {sup 96}Nb, {sup 124}Sb, and {sup 126}Sb produced by photofission of {sup 232}Th with 27-MeV peak bremsstrahlung and for {sup 136}Cs at 11, 15, and 27 MeV. Upper limits for the independent yields for {sup 86}Rb and {sup 134}Cs and mass yields for mass chains 125 and 127 were also measured for {sup 232}Th photofission at 27 MeV. Various extensions of the {ital Z}{sub {ital p}} charge-distribution model were found to give generally good agreement with experimental measurements in the asymmetric mass regions, but less satisfactory agreement in the symmetric region. A statistical charge-distribution model incorporating post-fission dynamics correlated well with experimental values in both symmetric and asymmetric regions. The statistical-dynamic model naturally predicted pairing and shell effects which were in good agreement with experimentally observed effects. One important outcome of the statistical-dynamic model calculations was the production of a linear shape on the wings of the charge-distribution curve when proximity proton transfer after scission was incorporated into the model. Such linear shapes have previously been experimentally observed without explanation.
OSTI ID:
5218441
Journal Information:
Physical Review, C (Nuclear Physics); (United States), Journal Name: Physical Review, C (Nuclear Physics); (United States) Vol. 44:3; ISSN 0556-2813; ISSN PRVCA
Country of Publication:
United States
Language:
English