Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Resonantly enhanced multiphoton ionization and third-harmonic generation in xenon gas

Journal Article · · Phys. Rev. Lett.; (United States)
Resonantly enhanced multiphoton ionization signals through the 6s(3/2)J=1 state of Xe rapidly disappear at pressures above 0.30 torr; concurrently, intense, vacuum-ultraviolet third-harmonic radiation is detected in the forward direction. Laser excitation spectra of the vacuum ultraviolet light exhibit increasing blue shifts and bandwidths with increasing pressure. The observed competition between ionization and third-harmonic generation is discussed in terms of a model involving fast collective emission.
Research Organization:
Chemical Physics Section, Health and Safety Research Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830
DOE Contract Number:
W-7405-ENG-26
OSTI ID:
5186930
Journal Information:
Phys. Rev. Lett.; (United States), Journal Name: Phys. Rev. Lett.; (United States) Vol. 45:2; ISSN PRLTA
Country of Publication:
United States
Language:
English