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Gas Production in the Photolysis of Liquid Methyl Iodide1

Journal Article · · Journal of the American Chemical Society
DOI:https://doi.org/10.1021/ja01111a056· OSTI ID:4368945
 [1];  [1]
  1. Canisius College, Buffalo, NY (United States)

The importance of ‘‘Hot Radical” processes in the photolysis of liquid methyl iodide is further evidenced in the formation of methane and ethane as gaseous products. For the reactions induced by light at 2537 A. the quantum yield for the formation of methane is 0.023, while that of ethane is 0.007. Although the iodine concentration is increasing during the course of the reaction, the ethane and methane yields are found to be independent of the extent of irradiation. The gas yields are dependent upon iodine concentration only at very high iodine concentrations. At room temperature, these yields are independent of the temperature of the sample. Methylene iodide is shown to be a product of the photolysis, while little or no hydrogen, ethylene, or acetylene formation is observed.

Research Organization:
Canisius College, Buffalo, NY (United States)
Sponsoring Organization:
US Atomic Energy Commission (AEC)
NSA Number:
NSA-07-002999
OSTI ID:
4368945
Report Number(s):
NYO--3263
Journal Information:
Journal of the American Chemical Society, Journal Name: Journal of the American Chemical Society Journal Issue: 15 Vol. 75; ISSN 0002-7863
Publisher:
American Chemical Society (ACS)Copyright Statement
Country of Publication:
United States
Language:
English

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