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THE COEFFICIENTS OF THE EQUILIBRIUM DISTRIBUTION OF DEUTERIUM IN ISOTOPIC EXCHANGE BETWEEN WATER AND SOME THIOLS (in Russian)

Journal Article · · Doklady Akad. Nauk S.S.S.R.
OSTI ID:4307804

>The equilibrium of deuterium exchange reactions between water and normal butylthiol, secondary butylthiol, isoamylthiol normal hexylihiol, and thiophenol was investigated. It was found that the isotopic equilibrium between the water and thiols is reached in 8 to 10 hr at 20 deg (in 2 hr in the exchange with thiophenol) and in 2 to 4 hr at 80 deg . In addition to direct exchange experiments (between deuterium enriched water and thiol with natural deuterium concentration) one reverse exchange experiment was made for each thiol at 20 deg . For these experiments water with natural concentration of deuterium and thiols was used, enriched, in previous direct exchange experiments, up to ~ 1%. The experiments confirmed the established thermodynamic equilibrium. (R.V.J.)

Research Organization:
Karpov Inst. of Physical Chemistry
NSA Number:
NSA-12-016267
OSTI ID:
4307804
Journal Information:
Doklady Akad. Nauk S.S.S.R., Journal Name: Doklady Akad. Nauk S.S.S.R. Vol. Vol: 121
Country of Publication:
Country unknown/Code not available
Language:
Russian

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