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Determination of the sign and magnitude of the nuclear quadrupole interaction by $beta$$-$$gamma$ directional correlations

Journal Article · · Phys. Rev., C, v. 12, no. 6, pp. 2022-2032
OSTI ID:4105022
Experiments are reported which demonstrate that the sign and magnitude of the quadrupole interaction of excited nuclear states can be reliably determined by means of time-differential $beta$$-$$gamma$ directional correlations with radioactive sources embedded in noncubic single crystals. The 828 keV level of $sup 115$In and the 247 keV level of $sup 111$Cd, fed by an allowed and a unique first-forbidden $beta$ decay, respectively, have been investigated by this method. The coupling constants e$sup 2$qQ of these levels in Cd metal at 298 degree K are: -146(5) MHz for $sup 115$In and +125(4) MHz for $sup 111$Cd. The positive coupling constant for $sup 111$Cd in Cd coupled with a positive quadrupole moment Q of this level implies a positive electric field gradient in Cd confirming recent theoretical predictions. The negative e$sup 2$qQ for the $sup 115$In level in Cd metal correspondingly indicates a negative Q for this level in conformity with its description as a member of a K = 1/2 rotational band. The paper includes a discussion of the major concepts underlying the various methods available now for determination of the sign of e$sup 2$qQ. Also, a detailed account of theoretical formulas necessary to evaluate allowed and forbidden $beta$$-$$gamma$ perturbed angular correlations and a brief discussion of the significance of the technique for further studies of nuclear quadrupole effects in materials are given. (AIP)
Research Organization:
Bell Laboratories, Murray Hill, New Jersey 07974
NSA Number:
NSA-33-019054
OSTI ID:
4105022
Journal Information:
Phys. Rev., C, v. 12, no. 6, pp. 2022-2032, Journal Name: Phys. Rev., C, v. 12, no. 6, pp. 2022-2032; ISSN PRVCA
Country of Publication:
United States
Language:
English