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U.S. Department of Energy
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REDUCTION OF PLUTONIUM(VI) TO PLUTONIUM(III) AND (IV) BY SODIUM NITRITE

Technical Report ·
DOI:https://doi.org/10.2172/4084403· OSTI ID:4084403

The use of anion exchange for final Pu purification in the Redox facility requires the adjustment of Pa(VI) to Pu(IV). Two methods of reduction were investigated: ferrous sulfamate and nitrite. The ferrous sulfamate method was adopted. Data on reduction of Pu(VI) to Pu(IV) and Pu(III) by nitrite are presented. The reduction by nitrite was found to be dependent on nitrite concentration, temperature, acidity, ferric ion concentration, and time, and it is possible to obtain >90% reduction to Pu(HI) by controlling the above conditions. (D.L.C.)

Research Organization:
General Electric Co. Hanford Atomic Products Operation, Richland, Wash.; Hanford Site (HNF), Richland, WA (United States)
Sponsoring Organization:
USDOE Office of Environmental Management (EM)
DOE Contract Number:
AT(45-1)-1350
NSA Number:
NSA-18-010038
OSTI ID:
4084403
Report Number(s):
HW-79354
Country of Publication:
United States
Language:
English