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Heteroepitaxy of strained and not-strained ferroelectric superlattices and their electric properties

Book ·
OSTI ID:392153
; ;  [1]
  1. Osaka Univ., Ibaraki, Osaka (Japan). Inst. for Scientific and Industrial Research

Bismuth based artificial superlattices have been formed by a layer-by-layer laser deposition with in-situ monitoring of RHEED. The Bi{sub 2}O{sub 2}/Wo{sub 6}, Bi2O{sub 2}/SrTa{sub 2}O{sub 9}, Bi{sub 2}O{sub 2}/SrTa{sub 2}O{sub 9}/SrTiO{sub 3} and Bi{sub 2}O{sub 2}/SrTa{sub 2}O{sub 9}/BaTiO{sub 3} are constructed epitaxially by a single, double and triple perovskite layers sandwiched by Bi{sub 2}O{sub 2} layers, respectively. The dielectric constant increases with increasing the number of perovskite layers. And the D-E hysteresis loop (ferroelectric properties) appears along the c-axis direction in odd perovskite layers (n = 1 and 3). The authors have also formed the SrTiO{sub 3}/BiWO{sub 6}/SrTiO{sub 3} multilayers. With this combination, the STO layers are isolated by the BWO layers. The dimensionality of STO layer can be controlled by changing the thickness of BWO layers. Below the BWO thickness of 500 {angstrom}, the {var_epsilon}{sub r} increases monotonously with decreasing the BWO thickness. Therefore, the coulomb force, which is in proportion to inverse of the distance, plays an essential role for the dielectric constant. The formation of artificially constructed ferroelectric films by a layer-by-layer deposition method will be discussed and an essential approach to elucidate the mechanism of ferroelectricity.

OSTI ID:
392153
Report Number(s):
CONF-951155--; ISBN 1-55899-304-5
Country of Publication:
United States
Language:
English