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Do dislocations and stacking faults increase the oxidation rate of pyrites?

Journal Article · · Geochimica et Cosmochimica Acta
; ; ;  [1];  [2];  [3]
  1. Pittsburgh Energy Technology Center, PA (United States)
  2. Univ. of California, San Diego, La Jolla, CA (United States)
  3. Sandia National Labs., Albuquerque, NM (United States)

XPS, SEM, and TEM studies were made on coal, non-coal, and shock-loaded pyrites that had been experimentally weathered under high relative humidity. Reactivity (oxidation) of the different pyrite samples may be related to their stacking fault densities. A coal pyrite sample that had the highest stacking fault concentration was also the most reactive pyrite. No systematic relationship between reactivity and dislocation density was observed. Shock-loaded samples exposed to mean bulk shock temperatures between 175 and 475{degrees}C showed an increase in the number of reactive sites and shock-loaded samples exposed to mean bulk shock temperatures between 500 and 700{degrees}C showed decreases in the number of reactive sites.

OSTI ID:
28580
Journal Information:
Geochimica et Cosmochimica Acta, Journal Name: Geochimica et Cosmochimica Acta Journal Issue: 21 Vol. 58; ISSN GCACAK; ISSN 0016-7037
Country of Publication:
United States
Language:
English